China is the world's largest cement-related mercury emitter. Atmospheric mercury inventories for China's cement industry are essential for appraising global mercury emissions and have been widely developed in previous studies associated with considerable uncertainties. In this study, we compiled high tempospatial resolution atmospheric mercury emission inventories for Chinese cement plants using the mass balance method and plantlevel input−output data. The effects of industry policies were investigated based on the inventories for 2007 and 2015. Nationwide emissions increased from 80 to 113 t due to rapid expansion of production and kiln-type substitution yet partly offset by policies involving capacity structure reformation. Pollution decreased in winter in northern China, thanks to the targeting policies. Mercury input, output, and storage in cement kilns in China were estimated. The uncertainty remarkably decreased relative to previous inventories. This study demonstrates the feasibility of establishing high-resolution emission inventories with the application of the mass balance method for all the individual plants nationwide and thus has implications for similar studies. This work also improves our understanding of the spatial patterns and temporal evolution of mercury emissions in China, thus offering references for the implementation of environment policies and the Minamata Convention on Mercury in China.
We propose a dust‐event detection and tracking procedure based on air quality data from the ground monitoring network by detecting temporal and spatial change‐points in PM10 concentration. It supplements the existing remote sensing based approach with high temporal resolution and better weather adaptivity. Applications of the procedure on the labeled data showed its having high discriminating power for dust events, pollution events, and clean periods. Our study finds changing correlation patterns between PM10 and other air pollutants at the start of the dust events, which are utilized to enhance the discriminating power of the dust‐event detection procedure. The detection and tracking procedure allows the construction of transport networks of the dust‐events as well as the identification of the source regions and the transportation pattern, and assess the intensity and severity of the dust‐events in North China. Our analysis find the dust‐events contributed to 23.3%–34.6% for PM10 and 18.2–33.2% for PM2.5 in the source regions and 2.0%–7.3% and 0.8%–4.0%, respectively, in the down‐stream provinces in the spring season from 2015 to 2020.
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