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Three-dimensionally ordered macroporous (3DOM) perovskite materials have attracted the interest from researchers worldwide due to their unique macroporous structure, flexible composition, tailorable physicochemical property, high stability and biocompatibility. In particular, they were widely used in environmental field, such as photocatalysis, catalytic combustion, catalytic oxidation and sensors. In this review, the recent progresses in the synthesis of 3DOM perovskite materials and their environmental applications are summarized. The advantages and the promoting mechanisms of 3DOM perovskite materials for different applications are discussed in detail. Subsequently, the challenges and perspectives on the topic are proposed.