The role of the metal-oxide interface in determining the spin polarization of electrons tunneling from or into ferromagnetic transition metals in magnetic tunnel junctions is reported. The spin polarization of cobalt in tunnel junctions with an alumina barrier is positive, but it is negative when the barrier is strontium titanate or cerium lanthanite. The results are ascribed to bonding effects at the transition metal-barrier interface. The influence of the electronic structure of metal-oxide interfaces on the spin polarization raises interesting fundamental problems and opens new ways to optimize the magnetoresistance of tunnel junctions.
Spin information processing is a possible new paradigm for post-CMOS
(complementary metal-oxide semiconductor) electronics and efficient spin
propagation over long distances is fundamental to this vision. However, despite
several decades of intense research, a suitable platform is still wanting. We
report here on highly efficient spin transport in two-terminal
polarizer/analyser devices based on high-mobility epitaxial graphene grown on
silicon carbide. Taking advantage of high-impedance injecting/detecting tunnel
junctions, we show spin transport efficiencies up to 75%, spin signals in the
mega-ohm range and spin diffusion lengths exceeding 100 {\mu}m. This enables
spintronics in complex structures: devices and network architectures relying on
spin information processing, well beyond present spintronics applications, can
now be foreseen
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