Particulate matter (PM) pollution from China is transported eastward to Korea and Japan and has been suggested to influence surface air quality on the West Coast of the United States. However, remote sensing studies have been inconclusive as to recent trends in Chinese emissions and transport. We reconciled different passive remote sensing points of view and found that while aerosol optical thickness (AOT) as an indicator of particulate pollution has increased from the start of the observation period (2000) to 2006–2007 from the main Chinese coastal outflow regions, since then there has been a 10–20% decrease in AOT (with respect to 2007). Reductions were observed in spring, summer, and fall seasons. No improvement in exported PM pollution is found for the winter season.

Abstract. Seven and a half years (June 2006 to November 2013) of Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) aerosol and cloud layer products are compared with collocated Ozone Monitoring Instrument (OMI) aerosol index (AI) data and Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) cloud products in order to investigate variability in estimates of biannual and monthly above-cloud aerosol (ACA) events globally. The active-(CALIOP) and passive-based (OMI-MODIS) techniques have their advantages and caveats for ACA detection, and thus both are used to derive a thorough and robust comparison of daytime cloudy-sky ACA distribution and climatology. For the first time, baseline above-cloud aerosol optical depth (ACAOD) and AI thresholds are derived and examined (AI = 1.0, ACAOD = 0.015) for each sensor. Both OMI-MODIS and CALIOP-based daytime spatial distributions of ACA events show similar patterns during both study periods (December-May) and (June-November). Divergence exists in some regions, however, such as Southeast Asia during June through November, where daytime cloudy-sky ACA frequencies of up to 10 % are found from CALIOP yet are non-existent from the OMI-based method. Conversely, annual cloudy-sky ACA frequencies of 20-30 % are reported over northern Africa from the OMI-based method yet are largely undetected by the CALIOP-based method. Using a collocated OMI-MODIS-CALIOP data set, our study suggests that the cloudy-sky ACA frequency differences between the OMI-MODIS-and CALIOP-based methods are mostly due to differences in cloud detection capability between MODIS and CALIOP as well as QA flags used. An increasing interannual variability of ∼ 0.3-0.4 % per year (since 2009) in global monthly cloudy-sky ACA daytime frequency of occurrence is found using the OMI-MODIS-based method. Yet, CALIOP-based global daytime ACA frequencies exhibit a near-zero interannual variability. Further analysis suggests that the OMI-derived interannual variability in cloudy-sky ACA frequency may be affected by OMI row anomalies in later years. A few regions are found to have increasing slopes in interannual variability in cloudysky ACA frequency, including the Middle East and India. Regions with slightly negative slopes of the interannual variability in cloudy-sky ACA frequencies are found over South America and China, while remaining regions in the study show nearly zero change in ACA frequencies over time. The interannual variability in ACA frequency is not, however, statistically significant on both global and regional scales, given the relatively limited sample sizes. A longer data record of ACA events is needed in order to establish significant trends of ACA frequency regionally and globally.

Using two different operational Aqua Moderate Resolution Imaging Spectroradiometer (MODIS)cloud optical depth (COD) retrievals (0.86 versus 1.6 μm), we evaluate the impact of above-cloud smoke aerosol particles on near-IR (0.86 μm) COD retrievals. Aerosol Index (AI) from the collocated Ozone Monitoring Instrument (OMI) are used to identify above-cloud aerosol particle loading over the southern Atlantic Ocean, including both smoke and dust from the African subcontinent. Collocated Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation data constrain cloud phase and provide contextual above-cloud aerosol optical depth. The frequency of occurrence of above-cloud aerosol events is depicted on a global scale for the spring and summer seasons from OMI and Cloud Aerosol Lidar with Orthogonal Polarization. Seasonal frequencies for smoke-over-cloud off the southwestern Africa coastline reach 20-50% in boreal summer. We find a corresponding low COD bias of 10-20% for standard MODIS COD retrievals when averaged OMI AI are larger than 1. No such bias is found over the Saharan dust outflow region off northern Africa, since both MODIS 0.86 and 1.6 μm channels are vulnerable to radiance attenuation due to dust particles. A similar result is found for a smaller domain, in the Gulf of Tonkin region, from smoke advection over marine stratocumulus clouds and outflow into the northern South China Sea in spring. This study shows the necessity of accounting for the above-cloud aerosol events for future studies using standard MODIS cloud products in biomass burning outflow regions, through the use of collocated OMI AI and supplementary MODIS 1.6 μm COD products.

Abstract. By combining Collection 6 Moderate Resolution and Imaging Spectroradiometer (MODIS) and Version 22 Multi-angle Imaging Spectroradiometer (MISR) aerosol products with Cloud and Earth's Radiant Energy System (CERES) flux products, the aerosol optical thickness (AOT, at 0.55 µm) and shortwave (SW) aerosol radiative effect (SWARE) trends are studied over ocean for the near-full Terra (2000Terra ( -2015 and Aqua (2002Aqua ( -2015 data records. Despite differences in sampling methods, regional SWARE and AOT trends are highly correlated with one another. Over global oceans, weak SWARE (cloud-free SW flux) and AOT trends of 0.5-0.6 W m −2 (−0.5 to −0.6 W m −2 ) and 0.002 AOT decade −1 are found using Terra data. Near-zero AOT and SWARE trends are also found for using Aqua data, regardless of the angular distribution models (ADMs) used. Regionally, positive AOT and cloud-free SW flux (negative SWARE) trends are found over the Bay of Bengal, the Arabian Sea, the Arabian/Persian Gulf and the Red Sea, while statistically significant negative trends are derived over the Mediterranean Sea and the eastern US coast. In addition, the global mean instantaneous SW aerosol direct forcing efficiencies are found to be ∼ −60 W m −2 AOT −1 , with corresponding SWARE values of ∼ −7 W m −2 from both Aqua and Terra data, again regardless of CERES ADMs used. Regionally, SW aerosol direct forcing efficiency values of ∼ −40 W m −2 AOT −1 are found over the southwest coast of Africa where smoke aerosol particles dominate in summer. Larger (in magnitude) SW aerosol direct forcing efficiency values of −50 to −80 W m −2 AOT −1 are found over several other dust-and pollutant-aerosol-dominated regions.Lastly, the AOT and SWARE trends from this study are also intercompared with aerosol trends (such as active-based ones) from several previous studies. Findings suggest that a cohesive understanding of the changing aerosol skies can be achieved through the analysis of observations from both passive-and active-based analyses, as well as from both narrowband and broadband datasets.

<p><strong>Abstract.</strong> By combining Collection 6 Moderate Resolution and Imaging Spectroradiometer (MODIS) and Version 22 Multi-angle Imaging Spectroradiometer (MISR) aerosol products with Cloud and Earth’s Radiant Energy System (CERES) flux products, the aerosol optical thickness (AOT, at 0.55 µm) and Short-Wave Aerosol Radiative Effect (SWARE) trends are studied over ocean for the near full Terra (2000–2015) and Aqua (2002–2015) data records. Despite differences in sampling methods, regional SWARE and AOT trends are highly correlated with one another. Over global oceans, weak SWARE (cloud free SW flux) and AOT trends of 0.5–0.6 W m<sup>−2</sup> (−0.5 to −0.6 W m<sup>−2</sup>) and 0.002 AOT decade<sup>−1</sup> were found using Terra data. Near zero AOT and SWARE trends are also found for using Aqua data, regardless of Angular Distribution Models (ADMs) used. Regionally, positive SWARE and AOT trends are found over the Bay of Bengal, Arabian Sea, Arabian/Persian Gulf and the Red Sea, while statistically significant negative trends are derived over the Mediterranean Sea and the eastern US coast. In addition, the global mean instantaneous SW aerosol direct forcing efficiencies are found to be ~ −60 W m<sup>−2</sup> per AOT, with corresponding SWARE values of ~ −7 W m<sup>−2</sup> from both Aqua and Terra data, and again, regardless of CERES ADMs used. Regionally, SW aerosol direct forcing efficiency values of ~ −40 W m<sup>−2</sup> per AOT are found over the southwest coast of Africa where smoke aerosol particles dominate in summer. Larger (in magnitude) SW aerosol direct forcing efficiency values of −50 to −80 W m<sup>−2</sup> per AOT are found over several other dust and pollutant aerosol dominated regions. Lastly, the AOT and SWARE trends from this study are also inter-compared with aerosol trends (such as active-based) from several previous studies. Findings suggest that a cohesive understanding of the changing aerosol skies can be achieved through the analysis of observations from both passive- and active-based analyses, as well as at both narrow-band and broad-band data sets.</p>