The antineutrino and electron spectra associated with various nuclear fuels are calculated. While there are substantial differences between the spectra of different uranium and plutonium isotopes, the dependence on the energy and flux of the fission-inducing neutrons is very weak. The resulting spectra can be used for the calculation of the antineutrino and electron spectra of an arbitrary nuclear reactor at various stages of its refueling cycle. The sources of uncertainties in the spectrum are identified and analyzed in detail. The. exposure time dependence of the spectrum is also discussed. The averaged cross sections of the inverse neutron {3 decay, weak charged and neutral-current-induced deuteron disintegration, and the antineutrino-electron scattering are then evaluated using ·the resulting v.

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The biological effects of radionuclides that emit α particles are of considerable interest in view of their potential for therapy and their presence in the environment. The present work is a continuation of our ongoing effort to study the radiotoxicity of α-particle emitters in vivo using the survival of murine testicular sperm heads as the biological end point. Specifically, the relative biological effectiveness (RBE) of very low-energy α particles (3.2 MeV) emitted by 148 Gd is investigated and determined to be 7.4 ± 2.4 when compared to the effects of acute external 120 kVp X rays. This datum, in conjunction with our earlier results for 210 Po and 212 Pb in equilibrium with its daughters, is used to revise and extend the range of validity of our previous RBE-energy relationship for α particles emitted by tissue-incorporated radionuclides. The new empirical relationship is given by RBE α = 9.14 − 0.510 E α , where 3 < E α < 9 MeV. The validity of this empirical relationship is tested by determining the RBE of the prolific α-particle emitter 223 Ra (in equilibrium with its daughters) experimentally in the same biological model and comparing the value obtained experimentally with the predicted value. The resulting RBE values are 5.4 ± 0.9 and 5.6, respectively. This close agreement strongly supports the adequacy of the empirical RBE-E α relationship to predict the biological effects of α-particle emitters in Vivo.

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