The dismantling of structural objects during the decommissioning of nuclear facilities needs radioactive source characterisation for the planning of decommissioning strategies in compliance with the ALARA (as low as reasonably achievable) principle. The sources may arise from neutron activation of the structural components in the reactor core as well as contamination due to the radioactive release from the fuel occurred during normal operation or unplanned events in a nuclear power plant (NPP). In a pressurised heavy water reactor (PHWR), various in-core components are predominantly made of either zircaloy–2 or 4. The nuclides present as impurities in the zircaloy, playing a crucial role in the activity inventory due to neutron activation of those nuclides, which in turn determine the external gamma dose rate. The activity of the activation products depend on the neutron flux seen by the component, duration of irradiation and cooling period, half-lives of the daughter products and the amount of the impurities present in the structural components. To illustrate this, a guide tube made up of zircaloy–4 has been considered. A guide tube assembly is a part of the primary shut down system (PSS) which guides the movement of absorber elements in the upward and downward direction in the calandria. This study has identified and quantified the activity inventory in a guide tube at the end of the operation of the reactor using the ORIGEN2 code, and then estimated the associated external gamma dose rate using the FLUKA Monte Carlo code. The findings will help the management of radioactive waste, cost optimisation and collective dose budgeting during the decommissioning stage of a typical PHWR.
The external radiation exposure from an overhead plume containing gamma emitting radionuclides can contribute substantial dose to the ground receptor during normal operations as well as accidental release conditions of nuclear facilities. In order to estimate the effective dose conversion coefficients (DCCs) directly, a finite plume Monte Carlo model along with the reference phantom at the ground receptor location needs to be implemented. In the present study, a comprehensive simulation of radiation transport from the Gaussian plume source to the ICRP reference adult voxel phantoms (receptor) is carried out using the FLUKA Monte Carlo code. The organ absorbed doses as well as the effective DCCs of the adult reference phantom are computed for different meteorological parameters and downwind distances. To illustrate the application of this model, an overhead Gaussian plume containing two different gamma emitting radionuclides, 135Xe and 41Ar are considered. From these simulations, the ratio of the effective dose rate to the kerma rate are estimated as 0.6 Sv Gy−1 and 0.65 Sv Gy−1 for the exposure from 135Xe and 41Ar, respectively. This ratio is constant irrespective of the meteorological conditions and cloud models. Further results show that the effective DCCs as a function of the downwind distance vary by an order of magnitude for an unstable weather category; however, the variations are very small in the case of a stable category. This study demonstrates an accurate method for calculating the effective dose to the ground receptor from an external plume which can be further applied for any radionuclide under any meteorological condition.
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