Optical frequency combs [1,2,3] provide equidistant frequency markers in the infrared, visible and ultra-violet [4,5] and can link an unknown optical frequency to a radio or microwave frequency reference [6,7]. Since their inception frequency combs have triggered major advances in optical frequency metrology and precision measurements [6,7] and in applications such as broadband laser-based gas sensing [8] and molecular fingerprinting [9]. Early work generated frequency combs by intra-cavity phase modulation [10,11], while to date frequency combs are generated utilizing the comb-like mode structure of mode-locked lasers, whose repetition rate and carrier envelope phase can be stabilized [12]. Here, we report an entirely novel approach in which equally spaced frequency markers are generated from a continuous wave (CW) pump laser of a known frequency interacting with the modes of a monolithic high-Q microresonator [13] via the Kerr nonlinearity [14,15]. The intrinsically broadband nature of parametric gain enables the generation of discrete comb modes over a 500 nm wide span (≈ 70 THz) around 1550 nm without relying on any external spectral broadening. Optical-heterodyne-based measurements reveal that cascaded parametric interactions give rise to an optical frequency comb, overcoming passive cavity dispersion. The uniformity of the mode spacing has been verified to within a relative experimental precision of 7.3×10 −18 . In contrast to femtosecond mode-locked lasers[16] the present work represents an enabling step towards a monolithic optical frequency comb generator allowing significant reduction in size, cost and power consumption. Moreover, the present approach can operate at previously unattainable repetition rates [17] exceeding 100 GHz which are useful in applications where the access to individual comb modes is required, such as optical waveform synthesis [18], high capacity telecommunications or astrophysical spectrometer calibration [19].Optical microcavities [20] are owing to their long temporal and small spatial light confinement ideally suited for nonlinear frequency conversion, which has led to a dramatic improvement in the threshold of nonlinear optical light conversion [21]. In contrast to stimulated gain, parametric frequency conversion [22] does not involve coupling to a dissipative reservoir, is broadband as it does not rely on atomic or molecular resonances and constitutes a phase sensitive amplification process, making it uniquely suited for tunable frequency conversion. In the case of a material with inversion symmetry -such as silica -the non linear optical effects are dominated by the third order non linearity. The process is based on four-wave mixing among two pump photons (frequency ν P ) with a signal (ν S ) and idler photon (ν I ) and results in the emergence of (phase coherent) signal and idler sidebands from the vacuum fluctuations at the expense of the pump field (cf. Fig.1). The observation of parametric interactions requires two conditions to be satisfied. First momentum conservation...

The series of precisely spaced, sharp spectral lines that form an optical frequency comb is enabling unprecedented measurement capabilities and new applications in a wide range of topics that include precision spectroscopy, atomic clocks, ultracold gases, and molecular fingerprinting. A new optical frequency comb generation principle has emerged that uses parametric frequency conversion in high resonance quality factor (Q) microresonators. This approach provides access to high repetition rates in the range of 10 to 1000 gigahertz through compact, chip-scale integration, permitting an increased number of comb applications, such as in astronomy, microwave photonics, or telecommunications. We review this emerging area and discuss opportunities that it presents for novel technologies as well as for fundamental science.

Extremely narrow optical resonances in cold atoms or single trapped ions can be measured with high resolution. A laser locked to such a narrow optical resonance could serve as a highly stable oscillator for an all-optical atomic clock. However, until recently there was no reliable clockwork mechanism that could count optical frequencies of hundreds of terahertz. Techniques using femtosecond-laser frequency combs, developed within the past few years, have solved this problem. The ability to count optical oscillations of more than 1015 cycles per second facilitates high-precision optical spectroscopy, and has led to the construction of an all-optical atomic clock that is expected eventually to outperform today's state-of-the-art caesium clocks.