Abstract. Space borne infrared limb emission measurements by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) reveal the formation of a belt of polar stratospheric clouds (PSCs) of nitric acid trihydrate (NAT) particles over Antarctica in mid-June 2003. By mesoscale microphysical simulations we show that this sudden onset of NAT PSCs was caused by heterogeneous nucleation on ice in the cooling phases of large-amplitude stratospheric mountain waves over the Antarctic Peninsula and the Ellsworth Mountains. MIPAS observations of PSCs before this event show no indication for the presence of NAT clouds with volume densities larger than about 0.3 µm3/cm3 and radii smaller than 3 µm, but are consistent with supercooled droplets of ternary H2SO4/HNO3/H2O solution (STS). Simulations indicate that homogeneous surface nucleation rates have to be reduced by three orders of magnitude to comply with the observations.
Abstract. Polar stratospheric clouds (PSC) have been observed in early winter (December 2002) during the SOLVE II/Vintersol campaign, both from balloons carrying comprehensive instrumentation for measurements of chemical composition, size distributions, and optical properties of the particles, as well as from individual backscatter soundings from Esrange and Sodankylä. The observations are unique in the sense that the PSC particles seem to have formed in the early winter under synoptic temperature conditions and not being influenced by mountain lee waves. A sequence of measurements during a 5-days period shows a gradual change between liquid and solid type PSCs with the development of a well-known sandwich structure. It appears that all PSC observations show the presence of a background population of solid particles, occasionally mixed in with more optically dominating liquid particles. The measurements have been compared with results from a detailed microphysical and optical simulation of the formation processes. Calculated extinctions are in good agreement with SAGE-III measurements from the same period. Apparently the solid particles are controlled by the synoptic temperature history while the presence of liquid particles is controlled by the local temperatures at the time of observation. The temperature histories indicate that the solid particles are nucleated above the ice frost point, and a surface freezing mechanism for this is included in the model. Reducing the calculated freezing ratesCorrespondence to: N. Larsen (nl@dmi.dk) by a factor 10-20, the model is able to simulate the observed particle size distributions and reproduce observed HNO 3 gas phase concentrations.
[1] A detailed microphysical model has been used to simulate polar stratospheric clouds (PSC) formed in mountain leewaves over northern Scandinavia and observed in a balloonborne multi-instrument flight on 25 January 2000. The measurements show cloud layers of large solid particles with nitric acid trihydrate (NAT) compositions at relatively high temperatures and layers containing liquid particles with supercooled ternary solution compositions at very low temperatures. The same PSC particle layers have been observed several times during the 2 1/2 h flight, offering a nearly Lagrangian picture of the particle evolution. The applied PSC model describes homogeneous freezing of ice below the ice frost point and diffusion-limited nonequilibrium and size-dependent growth and composition of liquid and solid-phase particles. The microphysical box model calculations are performed on two isentropic surfaces, corresponding to different observed particle layers, using temperature histories from combined high-resolution nonhydrostatic mesoscale and synoptic-scale model analyses of the meteorological conditions characterized by strong mountain leewaves. The calculated particle composition, physical phase, and particle size distributions are compared with the in situ measurements of the same particle properties. It appears that homogeneous freezing of ice in liquid solutions a few degrees below the ice frost point and subsequent release of NAT at higher temperatures might explain the characteristics of the observed solid PSC particles.
The Greenland ice sheet is a major contributor to sea level rise, adding on average 0.47 ± 0.23 mm year − 1 to global mean sea level between 1991 and 2015. The cryosphere as a whole has contributed around 45% of observed global sea level rise since 1993. Understanding the present-day state of the Greenland ice sheet is therefore vital for understanding the processes controlling the modern-day rates of sea level change and for making projections of sea level rise into the future. Here, we provide an overview of the current state of the mass budget of Greenland based on a diverse range of remote sensing observations to produce the essential climate variables (ECVs) of ice velocity, surface elevation change, grounding line location, calving front location, and gravimetric mass balance as well as numerical modelling that together build a consistent picture of a shrinking ice sheet. We also combine these observations with output from a regional climate model and from an ice sheet model to gain insight into existing biases in ice sheet dynamics and surface mass balance processes. Observations show surface lowering across virtually all regions of the ice sheet and at some locations up to −2.65 m year − 1 between 1995 and 2017 based on radar altimetry analysis. In addition, calving fronts at 28 study sites, representing a sample of typical glaciers, have retreated all around Greenland since the 1990s and in only two out of 28 study locations have they remained stable. During the same period, two of five floating ice shelves have collapsed while the locations of grounding lines at the remaining three floating ice shelves have remained stable over the observation period. In a detailed case study with a fracture model at Petermann glacier, we demonstrate the potential sensitivity of these floating ice shelves to future warming. GRACE gravimetrically-derived mass balance (GMB) data shows that overall Greenland has lost 255 ± 15 Gt year − 1 of ice over the period 2003 to 2016, consistent with that shown by IMBIE and a marked increase compared to a rate of loss of 83 ± 63 Gt year − 1 in the 1993–2003 period. Regional climate model and ice sheet model simulations show that surface mass processes dominate the Greenland ice sheet mass budget over most of the interior. However, in areas of high ice velocity there is a significant contribution to mass loss by ice dynamical processes. Marked differences between models and observations indicate that not all processes are captured accurately within models, indicating areas for future research.
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