We have explored the spin liquid state in Tb(2)Ti(2)O(7) with vibrating-coil magnetometry down to ~0.04 K under magnetic fields up to 5 T. We observe magnetic history dependence below T*~0.2 K reminiscent of the classical spin ice systems Ho(2)Ti(2)O(7) and Dy(2)TiTi(2)O(7). The magnetic phase diagram inferred from the magnetization is essentially isotropic, without evidence of magnetization plateaus as anticipated for so-called quantum spin ice, predicted theoretically for [111] when quantum fluctuations renormalize the interactions. Instead, the magnetization for T≪T* agrees semiquantitatively with the predictions of "all-in-all-out" (AIAO) antiferromagnetism. Taken together, this suggests that the spin liquid state in Tb(2)Ti(2)O(7) is akin to an incipient AIAO antiferromagnet.
Systems lacking inversion symmetry, such as selected three-dimensional compounds, multilayers and surfaces support Dzyaloshinsky-Moriya (DM) spin-orbit interactions. In recent years DM interactions have attracted great interest, because they may stabilize magnetic structures with a unique chirality and non-trivial topology. The inherent coupling between the various properties provided by DM interactions is potentially relevant for a variety of applications including, for instance, multiferroic and spintronic devices. The, perhaps, most extensively studied material in which DM interactions are important is the cubic B20 compound MnSi. We review the magnetic field and pressure dependence of the magnetic properties of MnSi. At ambient pressure this material displays helical order. Under hydrostatic pressure a non-Fermi liquid state emerges, where a partial magnetic order, reminiscent of liquid crystals, is observed in a small pocket. Recent experiments strongly suggest that the non-Fermi liquid state is not due to quantum criticality. Instead it may be the signature of spin textures and spin excitations with a non-trivial topology.
We report vibrating coil magnetometry of the spin-ice system Ho(2)Ti(2)O(7) down to ~0.04 K for magnetic fields up to 5 T applied parallel to the [111] axis. History-dependent behavior emerges below T(0)(*) ~ 0.6 K near zero magnetic field, in common with other spin-ice compounds. In large magnetic fields, we observe a magnetization plateau followed by a hysteretic metamagnetic transition. The temperature dependence of the coercive fields as well as the susceptibility calculated from the magnetization identify the metamagnetic transition as a line of first order transitions terminating in a critical end point at T(m)(*) 0.37 ~/= K, B(m) ~/= 1.5 T. The metamagnetic transition in Ho(2)Ti(2)O(7) is strongly reminiscent of that observed in Dy(2)Ti(2)O(7), suggestive of a general feature of the spin ices.
The in-pile positron source NEPOMUC of the Munich research reactor FRM II delivers a low-energy positron beam of highest intensity. Different source potentials can be applied in order to vary the primary kinetic energy of the positrons in the range between 15 eV and 1 keV. The maximum yield of slow positrons is up to 4 × 10 7 and 5 × 10 8 moderated positrons per second, respectively. New instruments for beam diagnostics have been implemented for the determination of the positron intensity and for positron beam profile measurements. The long-term stability and the degradation of the platinum moderator as well as the recovery procedure were investigated. In the present arrangement of NEPOMUC's instrumentation the monoenergetic positron beam is magnetically guided to different experiments: a coincident Doppler broadening spectrometer (CDBS) and an analysis chamber for positron induced Auger electron spectroscopy (PAES). In addition, an apparatus for the production of the negatively charged positronium ion was connected to the beam line in order to investigate this bound leptonic system in collaboration with the Max-Planck Institute for nuclear physics. An overview of the beam performance, the current status of the positron beam facility and the experiments is presented.
We report the development of a vibrating coil magnetometer (VCM) as combined with a top-loading dilution refrigerator for measurements of the magnetization down to millikelvin temperatures. The VCM offers unique measurement conditions, notably efficient cooling of the sample, data collection in uniform magnetic fields, the possibility to study strong magnetic anisotropies, fast data collection over a very wide range of magnetic fields, and the possibility of fast sample changes. In first measurements of the dipolar Ising magnet LiHoF(4) we readily achieved an excellent long-term stability of the vibration drive system of the VCM providing a sensitivity in excess of 10(-4) emu.
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