[1] Analysis of the continuous and collocated measurements of columnar spectral aerosol optical depths (AODs) and mass size distributions in the marine atmospheric boundary layer (MABL) over the Bay of Bengal (BoB), carried out from 27 December 2008 to 29 January 2009 during the Winter Integrated Campaign for Aerosols, Gases and Radiation Budget (W-ICARB), revealed distinct regional features in the spatial variations of the aerosol properties in the MABL and column. In general, AODs were high over the northern and northwestern parts of the BoB, with pockets of very high values, within which the AODs were as high as ∼0.8 while the smallest values (∼0.1) were observed over the northeastern BoB, off the Myanmar and Bangladesh coasts. Interestingly, though, this region had the highest Angstrom wavelength exponent a (∼1.5), notwithstanding the generally high values that prevailed over the eastern as well as northern coastal regions of India. Back trajectory analyses revealed the significant role of the advected aerosols in the observed spatial pattern. Within the MABL, high accumulation mode mass concentrations (M A ) prevailed over the entire BoB with the accumulation fraction ranging from 0.6 to 0.95, whereas very high fine-mode (r < 0.1 mm) aerosol mass fractions (∼0.8) were observed over the northeastern and western coastal BoB adjoining the Indian mainland (where a was high to very high). The vertical distributions, inferred from the columnar and MABL properties as well as from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations data, revealed better homogeneity in the northeastern and eastern BoB, whereas significant heterogeneity was seen over other regions.
[1] We present the climatology of aerosol microphysics, its trends, and impact of potential sources based on the long term measurements (for a period of 11.5 years from December 2001 to May 2012) of aerosol optical depths (AOD) in the spectral range 340-1020 nm from an urban center Delhi (28.6 N, 77.3 E, 238 m mean sea level) in the western Indo-Gangetic Plain (IGP). The study is the first ever long-term characterization of aerosols over the western IGP from the ground-based measurements. AODs are known to affect the air quality, visibility, radiative balance, and cloud microphysics of the region and IGP is one of the highest populated and polluted regions of the world. Our measurements show consistently high AOD during the entire period of observation. The seasonal variations of spectral AODs and Angstrom parameters are generally consistent every year. The AODs show a weak but statistically significant (in 95% confidence level) decreasing trend approximately À0.02/year at 500 nm, possibly, modulated by the pre-monsoon heavy dust loading during the first half of the observation period. The climatological monthly mean AOD at shorter wavelengths peaks twice, during June and November, while at longer wavelengths it shows only one peak in June. The annual variations of Angstrom exponent, a and its derivative, a′ suggest the prevalence of multi-modal aerosol size distributions at Delhi. The coarse-mode aerosols dominate during summer (March-June) and monsoon (July-September) seasons, whereas fine/accumulation mode enhances during post-monsoon (October-November) and winter (December-February) seasons. Potential advection pathways have been identified using concentration weighted trajectory (CWT) analysis of the 5 day isentropic air mass back trajectories at the observation site and their seasonal variations are discussed.
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