Light-emitting sources and devices permeate every aspect of our lives and are used in lighting, communications, transportation, computing, and medicine. Advances in multifunctional and “smart lighting” would require revolutionary concepts in the control of emission spectra and directionality. Such control might be possible with new schemes and regimes of light–matter interaction paired with developments in light-emitting materials. Here we show that all-dielectric metasurfaces made from III–V semiconductors with embedded emitters have the potential to provide revolutionary lighting concepts and devices, with new functionality that goes far beyond what is available in existing technologies. Specifically, we use Mie-resonant metasurfaces made from semiconductor heterostructures containing epitaxial quantum dots. By controlling the symmetry of the resonant modes, their overlap with the emission spectra, and other structural parameters, we can enhance the brightness by 2 orders of magnitude, as well as reduce its far-field divergence significantly.
Quantum state engineering, the cornerstone of quantum photonic technologies, mainly relies on spontaneous parametric downconversion and four-wave mixing, where one or two pump photons spontaneously decay into a photon pair. Both of these nonlinear effects require momentum conservation for the participating photons, which strongly limits the versatility of the resulting quantum states. Nonlinear metasurfaces have subwavelength thickness and allow the relaxation of this constraint; when combined with resonances, they greatly expand the possibilities of quantum state engineering. Here, we generated entangled photons via spontaneous parametric downconversion in semiconductor metasurfaces with high–quality factor, quasi-bound state in the continuum resonances. By enhancing the quantum vacuum field, our metasurfaces boost the emission of nondegenerate entangled photons within multiple narrow resonance bands and over a wide spectral range. A single resonance or several resonances in the same sample, pumped at multiple wavelengths, can generate multifrequency quantum states, including cluster states. These features reveal metasurfaces as versatile sources of complex states for quantum information.
We report on the room temperature thermal conductivity of AlAs-GaAs superlattices (SLs), in which we systematically vary the period thickness and total thickness between 2 − 24 nm and 20.1 − 2,160 nm, respectively. The thermal conductivity increases with the SL thickness and plateaus at a thickness around 200 nm, showing a clear transition from a quasi-ballistic to a diffusive phonon transport regime. These results demonstrate the existence of classical size effects in SLs, even at the highest interface density samples. We use harmonic Atomistic Green's function calculations to capture incoherence in phonon transport by averaging the calculated transmission over several purely coherent simulations of independent SL with different random mixing at the AlAs-GaAs interfaces. These simulations demonstrate the significant contribution of incoherent phonon transport through the decrease in the transmission and conductance in the SLs as the number of interfaces increases. In spite of this conductance decrease, our simulations show a quasilinear increase in thermal conductivity with the superlattice thickness. This suggests that the observation of a quasilinear increase in thermal conductivity can have important contributions from incoherent phonon transport. Furthermore, this seemingly linear slope in thermal conductivity vs. SL thickness data may actually be non-linear when extended to a larger number of periods, which is a signature of incoherent effects. Indeed, this trend for superlattices with interatomic mixing at the interfaces could easily be interpreted as linear when the number of periods is small. Our results reveal that the change in thermal conductivity with period thickness is dominated by incoherent (particlelike) phonons, whose properties are not dictated by changes in the AlAs or GaAs phonon dispersion relations. This work demonstrates the importance of studying both period and sample thickness dependencies of thermal conductivity to understand the relative contributions of coherent and incoherent phonon transport in the thermal conductivity in SLs.
Perfect absorption of light by an optically thin metasurface is among several remarkable optical functionalities enabled by nanophotonics. This functionality can be introduced into optoelectronic devices by structuring an active semiconductor-based element as a perfectly absorbing all-dielectric metasurface, leading to improved optical properties while simultaneously providing electrical conductivity. However, a delicate combination of geometrical and material parameters is required for perfect absorption, and currently, no general all-dielectric metasurface design fulfills these conditions for a desired semiconductor and operation wavelength. Here, using numerical simulations, we demonstrate that Mie resonators with subwavelength-size interconnecting channels allow this combination of perfect absorption requirements to be satisfied for different wavelengths of operation and different levels of intrinsic material absorption. We reveal the underlying physics and show that interconnecting channels play a critical role in achieving perfect absorption through their effects on the resonant wavelengths and losses for the electric dipole and magnetic dipole modes in Mie resonators. By adjusting only the channel widths, perfect absorption can be achieved for an optically thin GaAs-based metasurface at a desired wavelength of operation in a range from 715 nm to 840 nm, where the intrinsic absorption level in GaAs varies by more than a factor of 2. Optical transmission experiments confirm that these metasurfaces resonantly enhance optical absorption. This work lays out the foundation and guidelines for replacing bulk semiconductors with electrically connected, optically thin, perfectly absorbing metasurfaces in optical detectors.
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