In
this study, we investigated the selective SO2 removal
performance of three absorbentsdistilled water (DW), aqueous
NaOH, and Na2SO3 solutionsfrom a typical
ship exhaust gas stream using a hollow-fiber membrane contactor. SEM
and contact angle analyses were performed to apprehend the morphological
and water interaction characteristics of the membrane. A SO2/CO2/N2 gas mixture (1000 ppm of SO2, 5.50 mol % CO2, balance N2) was used and
the absorbents were thoroughly evaluated in terms of SO2 gas removal efficiency over a range of operating parameters including
absorbent flow rate, feed gas flow rate, absorbent concentration,
and L/G ratio. The aq. NaOH absorbent had the best SO2 removal
efficiency among the three absorbents under all conditions, mainly
due to high alkalinity. Notably, around 100% SO2 removal
efficiency can be achieved with the NaOH absorbent. The Na2SO3 solution closely followed the NaOH in SO2 removal efficiency. DW was the worst performer under all conditions.
This study confirms that the use of membrane contactor is advantageous
over the conventional packed towers because the membrane contactors
are compact, offer high contact area, and achieve higher removal efficiencies.
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