We have investigated the spin dynamics of YMnO 3 by inelastic neutron scattering and determined the spin-wave dispersion at low temperature. The spin-wave dispersions at low temperature have been analyzed with a simple nearest-neighbor anisotropic Heisenberg model and also by an anisotropic Hubbard model. Best fits are obtained only in the strong-coupling limit ͑U / t Ͼ ϳ 15͒, with planar exchange energy J =4t 2 / U Ӎ 2.4 meV, and anisotropy terms D z = U x Ј − U z Ј Ӎ 0.32 meV and D y = U x Ј − U y Ј Ӎ 0.033 meV. We have shown that in the strong-coupling limit, the anisotropic Hubbard model maps into the anisotropic Heisenberg model.
A purely fermionic representation is introduced for the ferromagnetic Kondo lattice model which allows conventional diagrammatic tools to be employed to study correlation effects. Quantum 1/S corrections to magnon excitations are investigated using a systematic inverse-degeneracy expansion scheme which incorporates correlation effects in the form of self-energy and vertex corrections, while explicitly preserving the continuous spin-rotation symmetry. Magnon self-energy is studied in the full range of interaction strength, and shown to result in strong magnon damping and anomalous softening for zone boundary modes, which accounts for several zoneboundary anomalies observed in recent spin-wave measurements of ferromagnetic manganites.
Evolution of the hole spectral function along the Γ − (π, π) cut is studied in the antiferromagnetic state of the Hubbard model. The kink in the calculated hole dispersion, the sharp spectral-weight transfer between the branches, and the drastically suppressed coherent spectral weight near k = (0, 0), as observed recently in the high-resolution ARPES studies of cuprate antiferromagnets, are shown to be strongly enhanced by finite-U double-occupancy effects. Together with the anomalous spin-wave dispersion observed earlier in high-resolution neutron-scattering studies, the present study provides further evidence of a unified description of magnetic and electronic excitations in cuprate antiferromagnets in terms of the Hubbard model.
Evolution of the magnetic response function in the triangular-lattice Hubbard model is studied with interaction strength within a systematic inverse-degeneracy expansion scheme which incorporates self-energy and vertex corrections and explicitly preserves the spin-rotation symmetry. It is shown that at half filling the response function goes through a nearly dispersionless regime around K for intermediate coupling strength, before undergoing an inversion at strong coupling, resulting in maximum response at the K point, consistent with the expected 120 • AF instability.Effects of finite hole/electron doping on the magnetic response function are also examined.
As performance of van der Waals heterostructure devices is governed by the nanoscale thicknesses and homogeneity of their constituent mono-to few-layer flakes, accurate mapping of these properties with high lateral resolution becomes imperative. Spectroscopic ellipsometry is a promising optical technique for such atomically thin-film characterization due to its simplicity, noninvasive nature and high accuracy. However, the effective use of standard ellipsometry methods on exfoliated micron-scale flakes is inhibited by their tens-of-microns lateral resolution or slow data acquisition. In this work, we demonstrate a Fourier imaging spectroscopic micro-ellipsometry method with sub-5 μm lateral resolution and three orders-of-magnitude faster data acquisition than similar-resolution ellipsometers. Simultaneous recording of spectroscopic ellipsometry information at multiple angles results in a highly sensitive system, which is used for performing angstrom-level accurate and consistent thickness mapping on exfoliated mono-, bi-and trilayers of graphene, hexagonal boron nitride (hBN) and transition metal dichalcogenide (MoS 2 , WS 2 , MoSe 2 , WSe 2 ) flakes. The system can successfully identify highly transparent monolayer hBN, a challenging proposition for other characterization tools. The optical microscope integrated ellipsometer can also map minute thickness variations over a micron-scale flake, revealing its lateral inhomogeneity. The prospect of adding standard optical elements to augment generic optical imaging and spectroscopy setups with accurate in situ ellipsometric mapping capability presents potential opportunities for investigation of exfoliated 2D materials.
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