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Abstract. High-resolution modelling is needed to understand urban air quality and pollutant dispersion in detail. Recently, the PALM model system 6.0, which is based on large-eddy simulation (LES), was extended with the detailed Sectional Aerosol module for Large Scale Applications (SALSA) v2.0 to enable studying the complex interactions between the turbulent flow field and aerosol dynamic processes. This study represents an extensive evaluation of the modelling system against the horizontal and vertical distributions of aerosol particles measured using a mobile laboratory and a drone in an urban neighbourhood in Helsinki, Finland. Specific emphasis is on the model sensitivity of aerosol particle concentrations, size distributions and chemical compositions to boundary conditions of meteorological variables and aerosol background concentrations. The meteorological boundary conditions are taken from both a numerical weather prediction model and observations, which occasionally differ strongly. Yet, the model shows good agreement with measurements (fractional bias <0.67, normalised mean squared error <6, fraction of the data within a factor of 2 >0.3, normalised mean bias factor <0.25 and normalised mean absolute error factor <0.35) with respect to both horizontal and vertical distribution of aerosol particles, their size distribution and chemical composition. The horizontal distribution is most sensitive to the wind speed and atmospheric stratification, and vertical distribution to the wind direction. The aerosol number size distribution is mainly governed by the flow field along the main street with high traffic rates and in its surroundings by the background concentrations. The results emphasise the importance of correct meteorological and aerosol background boundary conditions, in addition to accurate emission estimates and detailed model physics, in quantitative high-resolution air pollution modelling and future urban LES studies.

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Abstract. High-resolution modelling is needed to understand urban air quality and pollutant dispersion in detail. Recently, the PALM model system 6.0, which is based on the large-eddy simulation (LES), was extended with a detailed aerosol module SALSA2.0 to enable studying the complex interactions between the turbulent flow field and aerosol dynamic processes. This study represents an extensive evaluation of the modelling system against the horizontal and vertical distributions of aerosol particles measured using a mobile laboratory and a drone in an urban neighbourhood in Helsinki, Finland. Specific emphasis is on the model sensitivity of aerosol particle concentrations, size distributions and chemical compositions to boundary conditions of meteorological variables and aerosol background concentrations. The meteorological boundary conditions are drawn from both a numerical weather prediction model and observations, which occasionally differ strongly. Yet, the model shows good agreement with measurements (fractional bias

Abstract. The structure of the urban boundary layer, and particularly the surface layer, displays significant complexity, which can be exacerbated by coastal effects for cities located in such regions. Resolving the complexity of the coastal urban boundary layer remains an important question for many applications such as air quality and numerical weather prediction. One of the most promising new techniques for measuring the structure of the surface layer is fibre-optic distributed temperature sensing (DTS), which has the potential to provide new significant insights for boundary layer meteorology by making it possible to study thermal turbulence with high spatial and temporal resolution. We present 14 weeks of profile measurements with a DTS system at an urban site in Helsinki, Finland, during the winter and spring of 2020. We assess the benefits and drawbacks of using DTS measurements to supplement sonic anemometry for longer measurement periods in varying meteorological conditions, including those found difficult for the DTS method in prior studies. Furthermore, we demonstrate the capabilities of the DTS system using two case scenarios: a study of the erosion of a near-ground cold layer during the passage of a warm front, and a comparison of the near-ground thermal structure with and without the presence of a sea-breeze cell during springtime convective boundary layer development. This study demonstrates the utility of DTS measurements in revealing the internal surface layer structure, beyond the predictions of traditional surface layer theories. This knowledge is important for improving surface layer theories and parametrisations, including those used in numerical weather prediction. The study also highlights the drawbacks of DTS measurements, caused by low signal-to-noise ratios in near-neutral atmospheric conditions, especially when such a system would be used to supplement turbulence measurements over longer periods. Overall, this study presents important considerations for planning new studies or ongoing measurements utilising this exciting and relatively new instrumentation.