We reveal that metasurfaces created by seemingly different lattices of (dielectric or metallic) meta-atoms with broken in-plane symmetry can support sharp high-Q resonances that originate from the physics of bound states in the continuum. We prove rigorously a direct link between the bound states in the continuum and the Fano resonances, and develop a general theory of such metasurfaces, suggesting the way for smart engineering of resonances for many applications in nanophotonics and meta-optics.Metasurfaces have attracted a lot of attention in the recent years due to novel ways for wavefront control, advanced light focusing, and ultra-thin optical elements [1]. Recently, metasurfaces based on high-index resonant dielectric materials [2] have emerged as essential building blocks for various functional meta-optics devices [3] due to their low intrinsic loss, with unique capabilities for controlling the propagation and localization of light. A key concept underlying the specific functionalities of many metasurfaces is the use of constituent elements with spatially varying optical properties and optical response characterized by high quality factors (Q factors) of the resonances.Many interesting phenomena have been shown for metasurfaces composed of arrays of meta-atoms with broken inplane inversion symmetry (see Fig. 1), which all demonstrate the excitation of high-Q resonances for the normal incidence of light. The examples are the demonstration of imagingbased molecular barcoding with pixelated dielectric metasurfaces [4] and manifestation of polarization-induced chirality in metamaterials [5], which both are composed of asymmetric pairs of tilted bars [see Fig. 1(a)], observation of trapped modes in arrays of dielectric nanodisks with asymmetric holes [6] [see Fig. 1(b)], sharp trapped-mode resonances in plasmonic and dielectric split-ring structures [7,8] [see, e.g., Fig. 1(c)], broken-symmetry Fano metasurfaces for enhanced nonlinear effects [9, 10] [see Fig. 1(d)], tunable high-Q Fano resonances in plasmonic metasurfaces [11] [see Fig. 1(e)], trapped light and metamaterial-induced transparency in arrays of square split-ring resonators [12,13] presented in Fig. 1(f). Here, we demonstrate that all such seemingly different structures can be unified by a general concept of bound states in the continuum, and we prove rigorously their link to the Fano resonances.Bound states in the continuum (BICs) originated from quantum mechanics as a curiosity [14], but later they were rediscovered as an important physical concept of destructive interference [15] being then extended to other fields of wave physics, including acoustics [16] and optics [17,18]. A true BIC is a mathematical object with an infinite Q factor and vanishing resonance width, it can exist only in ideal lossless infinite structures or for extreme values of parameters [19][20][21]. In practice, BIC can be realized as a quasi-BIC in the form of a supercavity mode [22] when both Q factor and resonance width become finite at the BIC conditions due to ab-d c a...
All-dielectric nanophotonics is an exciting and rapidly developing area of nanooptics which utilizes the resonant behavior of high-index low-loss dielectric nanoparticles for enhancing light-matter interaction on the nanoscale. When experimental implementation of a specific all-dielectric nanostructure is an issue, two crucial factors have to be in focus: the choice of a high-index material and a fabrication method. The degree to which various effects can be enhanced relies on the dielectric response of the chosen material as well as the fabrication accuracy. Here, we make an overview of available high-index materials and existing fabrication techniques for the realization of all-dielectric nanostructures. We compare performance of the chosen materials in the visible and IR spectral ranges in terms of scattering efficiencies and Q-factors. Various fabrication methods of all-dielectric nanostructures are further discussed, and their advantages and disadvantages are highlighted. We also present an outlook for the search of better materials with higher refractive indices and novel fabrication methods enabling low-cost manufacturing of optically resonant high-index nanoparticles. We hope that our results will be valuable for researches across the whole field of nanophotonics and particularly for the design of all-dielectric nanostructures.
Two-dimensional semiconducting transition metal dichalcogenides (TMDCs) are extremely attractive materials for optoelectronic applications in the visible and near-infrared range. Coupling these materials to optical nanocavities enables advanced quantum optics and nanophotonic devices. Here, we address the issue of resonance coupling in hybrid exciton-polariton structures based on single Si nanoparticles (NPs) coupled to monolayer (1L)-WS. We predict a strong coupling regime with a Rabi splitting energy exceeding 110 meV for a Si NP covered by 1L-WS at the magnetic optical Mie resonance because of the symmetry of the mode. Further, we achieve a large enhancement in the Rabi splitting energy up to 208 meV by changing the surrounding dielectric material from air to water. The prediction is based on the experimental estimation of TMDC dipole moment variation obtained from the measured photoluminescence spectra of 1L-WS in different solvents. An ability of such a system to tune the resonance coupling is realized experimentally for optically resonant spherical Si NPs placed on 1L-WS. The Rabi splitting energy obtained for this scenario increases from 49.6 to 86.6 meV after replacing air by water. Our findings pave the way to develop high-efficiency optoelectronic, nanophotonic, and quantum optical devices.
Two-dimensional semiconducting transition metal dichalcogenides (TMDCs) have recently become attractive materials for several optoelectronic applications, such as photodetection, light harvesting, phototransistors, light-emitting diodes, and lasers. Their bandgap lies in the visible and near-IR range, and they possess strong excitonic resonances, high oscillator strengths, and valley-selective response. Coupling these materials to optical nanocavities enhances the quantum yield of exciton emission, enabling advanced quantum optics and nanophotonics devices. Here, we review the state-of-the-art advances of hybrid exciton-polariton structures based on monolayer TMDCs coupled to plasmonic and dielectric nanocavities. We discuss the optical properties of 2D WS, WSe, MoS and MoSe materials, paying special attention to their energy bands, photoluminescence/absorption spectra, excitonic fine structure, and to the dynamics of exciton formation and valley depolarization. We also discuss light-matter interactions in such hybrid exciton-polariton structures. Finally, we focus on weak and strong coupling regimes in monolayer TMDCs-based exciton-polariton systems, envisioning research directions and future opportunities for this material platform.
Photoconductive antennas are promising sources of terahertz radiation that is widely used for spectroscopy, characterization, and imaging of biological objects, deep space studies, scanning of surfaces, and detection of potentially hazardous substances. These antennas are compact and allow for generation of both ultrabroadband pulses and tunable continuous wave terahertz signals at room temperatures, with no need for high‐power optical sources. However, such antennas have relatively low energy conversion efficiency of femtosecond laser pulses or two close pump wavelengths (photomixers) into the pulsed and continuous terahertz radiation, correspondingly. Recently, an approach to solving this problem that involves known methods of nanophotonics applied to terahertz photoconductive antennas and photomixers has been proposed. This approach comprises the use of optical nanoantennas for enhancing the absorption of pump laser radiation in the antenna gap, reducing the lifetime of photoexcited carriers, and improving the antenna thermal efficiency. This Review is intended to systematize the main results obtained by researchers in this promising field of hybrid optical‐to‐terahertz photoconductive antennas and photomixers. We summarize the main results on hybrid THz antennas, compare the approaches to their implementation, and offer further perspectives of their development including an application of all‐dielectric nanoantennas instead of plasmonic ones.
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