To generate a radially polarized laser beam we designed and fabricated a new Brewster optical element that consists of convex and concave conical prisms. The lateral surface of the convex conical prism was coated with a dielectric multilayer (SiO2 and Ta2O5) to enhance polarization selectivity. By combining two prisms we obtained a conical Brewster prism without beam divergence owing to refraction. A radially polarized TEM01* (R-TEM01*) mode laser beam was demonstrated when this prism was used inside a Nd:YAG laser cavity.

Gold particles were fabricated by the high-intensity femtosecond laser irradiation of gold (III) chloride trihydrate (HAuCl4) aqueous solution. The structure and size distribution of the prepared particles were evaluated by transmission electron microscopy. The configuration of the gold particles varied with the concentration of the HAuCl4 aqueous solution. The mean particle size and size distribution were changed by the addition of polyvinylpyrrolidone (PVP), which acted as a dispersant, and monodispersed gold nanoparticles with a diameter of about 3 nm were successfully fabricated. The formation process of the nanoparticles is discussed in terms of the optical decomposition of molecules in the highly intense optical field generated by femtosecond laser irradiation.

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The intensity distributions near the focal point for radially polarized laser beams including higher-order transverse modes are calculated based on vector diffraction theory. For higher-order radially polarized mode beams as well as a fundamental mode (R-TEM01*) beam, the strong longitudinal component forms a sharper spot at the focal point under a high-NA focusing condition. In particular, double-ring-shaped radially polarized mode (R-TEM11*) beams can effectively reduce the focal spot size because of destructive interference between the inner and the outer rings with pi phase shift. Compared with an R-TEM01* beam focusing in a limit of NA=1, the full width at half-maximum values of the focal spot for an R-TEM11* beam are decreased by 13.6% for the longitudinal component and 25.8% for the total intensity.

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