We report a free-surface electrohydrodynamic flow phenomenon driven by an ionic wind mechanism induced by a high frequency gas-phase ac field ͑Ͼ10 kHz͒. Intense vortices Ͼ1 cm/s are generated above a critical voltage, beyond which the vortices break down to spawn off new vortex pairs leading to a cascade of vortices over a continuum of length scales; the mixing efficiency approaches a turbulent-like state. Colloidal particles are attracted and aggregated into planar crystal structures within the vortices by a combination of dielectrophoresis and shear-induced diffusion.