Large variations in the growth of atmospheric methane, a prominent greenhouse gas, are driven by a diverse range of anthropogenic and natural emissions and by loss from oxidation by the hydroxyl radical. We used a decade-long dataset (2010–2019) of satellite observations of methane to show that tropical terrestrial emissions explain more than 80% of the observed changes in the global atmospheric methane growth rate over this period. Using correlative meteorological analyses, we show strong seasonal correlations (r = 0.6–0.8) between large-scale changes in sea surface temperature over the tropical oceans and regional variations in methane emissions (via changes in rainfall and temperature) over tropical South America and tropical Africa. Existing predictive skill for sea surface temperature variations could therefore be used to help forecast variations in global atmospheric methane.
Space-borne measurements of atmospheric greenhouse gas concentrations provide global observation constraints for top-down estimates of surface carbon flux. Here, the first estimates of the global distribution of carbon surface fluxes inferred from dry-air CO 2 column (XCO 2 ) measurements by the Chinese Global Carbon Dioxide Monitoring Scientific Experimental Satellite (TanSat) are presented. An ensemble transform Kalman filter (ETKF) data assimilation system coupled with the GEOS-Chem global chemistry transport model is used to optimally fit model simulations with the TanSat XCO 2 observations, which were retrieved using the Institute of Atmospheric Physics Carbon dioxide retrieval Algorithm for Satellite remote sensing (IAPCAS). High posterior error reduction (30%-50%) compared with a priori fluxes indicates that assimilating satellite XCO 2 measurements provides highly effective constraints on global carbon flux estimation. Their impacts are also highlighted by significant spatiotemporal shifts in flux patterns over regions critical to the global carbon budget, such as tropical South America and China. An integrated global land carbon net flux of 6.71 ± 0.76 Gt C yr −1 over 12 months (May 2017-April 2018) is estimated from the TanSat XCO 2 data, which is generally consistent with other inversions based on satellite data, such as the JAXA GOSAT and NASA OCO-2 XCO 2 retrievals. However, discrepancies were found in some regional flux estimates, particularly over the Southern Hemisphere, where there may still be uncorrected bias between satellite measurements due to the lack of independent reference observations. The results of this study provide the groundwork for further studies using current or future TanSat XCO 2 data together with other surfacebased and space-borne measurements to quantify biosphere-atmosphere carbon exchange.
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