Strong coupling between a cavity and transition dipole moments in emitters leads to vacuum Rabi splitting. Researchers have not reported strong coupling between a single emitter and a dielectric cavity at room temperature until now. In this study, we investigated the photoluminescence (PL) spectra of colloidal quantum dots on the surface of a SiO2/Si material at various collection angles at room temperature. We measured the corresponding reflection spectra for the SiO2/Si material and compared them with the PL spectra. We observed PL spectral splitting and regarded it as strong coupling between colloidal quantum dots and the SiO2/Si material. Upper polaritons and lower polaritons exhibited anticrossing behavior. We observed Rabi splitting from single-photon emission in the dielectric cavity at room temperature. Through analysis, we attributed the Rabi splitting to strong coupling between quantum dots and bound states in the continuum in the low-refractive-index/high-refractive-index hybrid material.
The interaction between light and matter has always been the focus of quantum science, and the realization of truly strong coupling between an exciton and the optical cavity is a basis of quantum information systems. As a special semiconductor material, colloidal quantum dots have fascinating optical properties. In this study, the photoluminescence spectra of colloidal quantum dots are measured at different collection angles in microcavities based on hybrid refractive-index waveguides. The photon bound states in the continuum are found in the low–high–low refractive-index hybrid waveguides in the appropriate waveguide width region, where the photoluminescence spectra of colloidal quantum dots split into two or more peaks. The upper polaritons and lower polaritons avoid resonance crossings in the systems. The Rabi splitting energy of 96.0 meV can be obtained. The observed phenomenon of vacuum Rabi splitting at room temperature is attributed to the strong coupling between quantum dots and the bound states in the continuum.
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