Methylsulfanyl derivatives of cobalt bis(dicarbollide), [8,

Stable imidates 10-EtC(OR)HN-7,8-C2B9H11 and thioimidates 10-EtC(SR)HN-7,8-C2B9H11 were synthesized via the reactions of a nitrilium derivative of nido-carborane 10-EtCN-7,8-C2B9H11 with alcohols and thiols.

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A number of new nido-carboranyl amidines 10-R(CH2)nNHC(Et)=HN-7,8-C2B9H11 (n = 2, R = OH, OMe, NMe2; n = 3, R = OH) were synthesized by nucleophilic addition of amino alcohols and...