NWs dispersed on SiO 2 generally exhibit much weaker luminescence (up to 10-3 times)
Quantum dots enable strong carrier confinement and exhibit a delta-function like density of states, offering significant improvements to laser performance and high-temperature stability when used as a gain medium. However, quantum dot lasers have been limited to photonic cavities that are diffraction-limited and further miniaturization to meet the demands of nanophotonic-electronic integration applications is challenging based on existing designs. Here we introduce the first quantum dot-based plasmonic laser to reduce the cross-sectional area of nanowire quantum dot lasers below the cutoff limit of photonic modes while maintaining the length in the order of the lasing wavelength. Metal organic chemical vapor deposition grown GaAs-AlGaAs core-shell nanowires containing InGaAs quantum dot stacks are placed directly on a silver film, and lasing was observed from single nanowires originating from the InGaAs quantum dot emission into the low-loss higher order plasmonic mode. Lasing threshold pump fluences as low as ∼120 μJ/cm(2) was observed at 7 K, and lasing was observed up to 125 K. Temperature stability from the quantum dot gain, leading to a high characteristic temperature was demonstrated. These results indicate that high-performance, miniaturized quantum dot lasers can be realized with plasmonics.
We report on the fabrication, nanomanipulation, and optical properties of ZnO-nanowire-induced nanocavities in grooved SiN photonic crystals. We show that subwavelength ZnO nanowires supporting intrinsically no Fabry−Peŕot mode in the violet and near-ultraviolet range can induce optical confinement when introduced in a grooved twodimensional photonic crystal waveguide. Despite fabrication challenges arising at such short wavelengths, this hybrid approach leads to fundamental nanocavity modes with resolution-limited quality factors larger than Q exp = 2.1 × 10 3 at λ = 403 nm for a mode volume V m = 5.9(λ/n r NW ) 3 = 3.4(λ/n r SiN ) 3 , as deduced from three-dimensional finite-difference timedomain calculations. The investigation of optical losses in our system shows that at wavelengths shorter than λ = 390 nm Q exp is limited by self-absorption, indicating a good nanowire to cavity coupling. These results validate our hybrid approach as an efficient way to circumvent the processing issues that were so far preventing the insertion of ZnO emitters in photonic crystal nanocavities. Furthermore, we demonstrate that the degree of freedom along the groove can be used to move nanowire-induced nanocavities in space, position them deterministically, and tune their optical properties in the near-ultraviolet range. This striking feature opens the path toward the realization of versatile nanophotonic devices including movable and tunable all-dielectric NW nanolasers operating at high temperature.
We compare the quality factor values of the whispering gallery modes of microdisks (μ-disks) incorporating GaN quantum dots (QDs) grown on AlN and AlGaN barriers by performing room temperature photoluminescence (PL) spectroscopy. The PL measurements show a large number of high Q factor resonant modes on the whole spectrum, which allows us to identify the different radial mode families and to compare them with simulations. We report a considerable improvement of the Q factor, which reflects the etching quality and the relatively low cavity loss by inserting QDs into the cavity. GaN/AlN QDs-based μ-disks show very high Q values (Q>7000) whereas the Q factor is only up to 2000 in μ-disks embedding QDs grown on the AlGaN barrier layer. We attribute this difference to the lower absorption below bandgap for AlN barrier layers at the energies of our experimental investigation.
We report the demonstration of single-photon emission from cubic GaN/AlN quantum dots grown by molecular beam epitaxy. We have observed spectrally clean and isolated emission peaks from these quantum dots. Clear single-photon emission was detected by analyzing one such peak at 4 K. The estimated g(2)[0] value is 0.25, which becomes 0.05 when corrected for background and detector dark counts. We have also observed the single-photon nature of the emission up to 100 K (g(2)[0] = 0.47). These results indicate that cubic GaN quantum dots are possible candidates for high-temperature operating UV single-photon sources with the possibility of integration into photonic nanostructures.
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