Femtosecond synchrotron pulses were generated directly from an electron storage ring. An ultrashort laser pulse was used to modulate the energy of electrons within a 100-femtosecond slice of the stored 30-picosecond electron bunch. The energy-modulated electrons were spatially separated from the long bunch and used to generate approximately 300-femtosecond synchrotron pulses at a bend-magnet beamline, with a spectral range from infrared to x-ray wavelengths. The same technique can be used to generate approximately 100-femtosecond x-ray pulses of substantially higher flux and brightness with an undulator. Such synchrotron-based femtosecond x-ray sources offer the possibility of applying x-ray techniques on an ultrafast time scale to investigate structural dynamics in condensed matter.

Pulses of x-rays 300 femtoseconds in duration at a wavelength of 0.4 angstroms (30,000 electron volts) have been generated by 90° Thomson scattering between infrared terawatt laser pulses and highly relativistic electrons from an accelerator. In the right-angle scattering geometry, the duration of the x-ray burst is determined by the transit time of the laser pulse across the ∼90-micrometer waist of the focused electron beam. The x-rays are highly directed (∼0.6° divergence) and can be tuned in energy. This source of femtosecond x-rays will make it possible to combine x-ray techniques with ultrafast time resolution to investigate structural dynamics in condensed matter.

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