No abstract

The angular distribution of bremsstrahlung gamma rays produced by fast electrons accelerated in relativistic laser-solid interaction has been studied by photoneutron activation in copper. We show that the gamma-ray beam moves from the target normal to the direction of the k(laser) vector as the scale length is increased. Similar behavior is found also in 2D particle-in-cell simulations.

The photodissociation of nitrobenzene and the nitrotoluene isomers at 375 nm, induced by a 90 femtosecond laser, is analyzed and compared with the fragmentation by a 10 nanosecond laser at the same wavelength. The molecular ionization is attributed to a nonresonant multiphoton process, and the observed fragmentation can be explained predominantly by an above ionization mechanism (ladder climbing). The mass spectra of the three nitrotoluene isomers show differences which can be used for analytical purposes. The molecular rearrangement taking place prior to the dissociation is also discussed. For nitrobenzene, it is suggested that most of the dissociation occurs from the nitrobenzene structure rather than that of phenyl nitrite. In the case of o-nitrotoluene, it seems that the hydrogen transfer from the -CH 3 to the NO 2 group (ortho effect) is favored in ionic states, while the rearrangement to a nitrite structure is possible in the excited electronic states.

A tuneable ultra-compact high-power, ultra-short pulsed, bright gamma-ray source based on bremsstrahlung radiation from laser-plasma accelerated electrons Novel measurements of electromagnetic radiation above 10 MeV are presented for ultra intense laser pulse interactions with solids. A bright, highly directional source of ␥ rays was observed directly behind the target. The ␥ rays were produced by bremsstrahlung radiation from energetic electrons generated during the interaction. They were measured using the photoneutron reaction ͓ 63 Cu(␥,n) 62 Cu͔ in copper. The resulting activity was measured by coincidence counting the positron annihilation ␥ rays which were produced from the decay of 62 Cu. New measurements of the bremsstrahlung radiation at 10 19 W cm Ϫ2 are also presented.

When a laser pulse of intensity 10(19) W cm(-2) interacts with solid targets, electrons of energies of some tens of MeV are produced. In a tantalum target, the electrons generate an intense highly directional gamma-ray beam that can be used to carry out photonuclear reactions. The isotopes 11C, 38K, (62,64)Cu, 63Zn, 106Ag, 140Pr, and 180Ta have been produced by (gamma,n) reactions using the VULCAN laser beam. In addition, laser-induced nuclear fission in 238U has been demonstrated, a process which was theoretically predicted at such laser intensities more than ten years ago. The ratio of the 11C and the 62Cu beta(+) activities yields shot-by-shot temperatures of the suprathermal electrons at laser intensities of approximately 10(19) W cm(-2).