The generation of significant photocurrents observed in plasmonic metasurfaces is interesting from a fundamental point of view and promising for applications in plasmon-based electronics and plasmonic sensors with compact electrical detection. We show that photoinduced voltages in strongly modulated plasmonic surfaces demonstrate a highly asymmetric angular dependence with polarity switching around the plasmon resonance conditions. The effects are tentatively attributed to coupling between localized and propagating plasmons.

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Giant enhancement of photocurrents in plasmonic structures (plasmon drag effect) provides opportunities for compact electric monitoring of plasmonic effects, and thus is promising for plasmonic-based sensing applications. In the experiment, we measure photoinduced electric signals in flat and profile-modulated systems, and test their sensitivity to small changes of the local dielectric environment, such as a presence of Langmuir–Blodgett monolayers at the metal surface. We show that the addition of a stearic acid monolayer leading to a small shift in plasmon resonance conditions can be ultimately resolved with electrical measurements as the switching in the photovoltage polarity.

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