Abstract. The seasonal and spatial variations of vertical distribution and optical properties of aerosols over China are studied using long-term satellite observations from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and ground-based lidar observations and Aerosol Robotic Network (AERONET) data. The CALIOP products are validated using the ground-based lidar measurements at the Semi-Arid Climate and Environment Observatory of Lanzhou University (SACOL). The Taklamakan Desert and Tibetan Plateau regions exhibit the highest depolarization and color ratios because of the natural dust origin, whereas the North China Plain, Sichuan Basin and Yangtze River Delta show the lowest depolarization and color ratios because of aerosols from secondary formation of the anthropogenic origin. Certain regions, such as the North China Plain in spring and the Loess Plateau in winter, show intermediate depolarization and color ratios because of mixed dust and anthropogenic aerosols. In the Pearl River Delta region, the depolarization and color ratios are similar to but higher than those of the other polluted regions because of combined anthropogenic and marine aerosols. Long-range transport of dust in the middle and upper troposphere in spring is well captured by the CALIOP observations. The seasonal variations in the aerosol vertical distributions reveal efficient transport of aerosols from the atmospheric boundary layer to the free troposphere because of summertime convective mixing. The aerosol extinction lapse rates in autumn and winter are more positive than those in spring and summer, indicating trapped aerosols within the boundary layer because of stabler meteorological conditions. More than 80 % of the column aerosols are distributed within 1.5 km above the ground in winter, when the aerosol extinction lapse rate exhibits a maximum seasonal average in all study regions except for the Tibetan Plateau. The aerosol extinction lapse rates in the polluted regions are higher than those of the less polluted regions, indicating a stabilized atmosphere due to absorptive aerosols in the polluted regions. Our results reveal that the satellite and ground-based remote-sensing measurements provide the key information on the long-term seasonal and spatial variations in the aerosol vertical distribution and optical properties, regional aerosol types, long-range transport and atmospheric stability, which can be utilized to more precisely assess the direct and indirect aerosol effects on weather and climate.

A multiplatform data set from the Clouds, Aerosol, and Precipitation in the Marine Boundary Layer (MBL) Graciosa, Azores, 2009-2010 field campaign was used to investigate how continental aerosols can influence MBL cloud condensation nuclei (CCN) number concentration (N CCN ). The seasonal variations of aerosol properties have shown that the winter and early spring months had the highest mean surface wind speed (> 5 m s À1) and greatest contribution of sea salt to aerosol optical depth (AOD), while continental fine mode aerosols were the main contributors to AOD during the warm season months (May-September). Five aerosol events consisting of mineral dust, pollution, biomass smoke, and volcanic ash particles were selected as case studies using Atmospheric Radiation Measurement (ARM) mobile facility measurements. The aerosols in Case I were found to primarily consist of coarse mode, Saharan mineral dust. For Case II, the aerosols were also coarse mode but consisted of volcanic ash. Case III had fine mode biomass smoke and pollution aerosol influences while Cases IV and V consisted of mixtures of North American pollution and Saharan dust that was advected by an extratropical cyclone to the Azores. Cases I, IV, and V exhibited weak correlations between aerosol loading and N CCN due to mineral dust influences, while Cases II and III had a strong relationship with N CCN likely due to the sulfate content in the volcanic ash and pollution particles. The permanent Eastern North Atlantic ARM facility over the Azores will aid in a future long-term study of aerosol effects on N CCN .

Asian aerosols are among the most complex yet widely studied components of the atmosphere not only due to their seasonal variability but also their effects on climate change. Four Aerosol Robotic Network (AERONET) sites have been selected to represent aerosol properties dominated by pollution (Taihu), mixed complex particle types (Xianghe), desert-urban (SACOL), and biomass (Mukdahan) in East Asia during the 2001–2010 period. The volume size distribution, aerosol optical depth (τ and &tau;_abs), Ångström exponent (α and &alpha;_abs), and the single scattering co-albedo (&omega;_oabs) parameters over the four selected sites have been used to (a) illustrate seasonal changes in aerosol size and composition and (b) discern the absorptive characteristics of black carbon (BC), organic carbon (OC), mineral dust particles, and mixtures. A strongly absorbing mineral dust influence is seen at the Xianghe, Taihu, and SACOL sites during the spring months (MAM), as given by coarse mode dominance, mean &alpha;_{440&ndash;870} < 1, and mean &alpha;_{abs440&ndash;870} > 1.5. There is a shift towards weakly absorbing pollution (sulfate) and biomass (OC) aerosol dominance in the summer (JJA) and autumn (SON) months, as given by a strong fine mode influence, &alpha;_{440&ndash;870} > 1, and &alpha;_{abs440&ndash;870} < 1.5. A winter season (DJF) shift toward strongly fine mode, absorbing particles (BC and OC) is observed at Xianghe and Taihu (&alpha;_{abs440&ndash;870} > 1 and &alpha;_{abs440&ndash;870} > 1.5). At Mukdahan, a strong fine mode influence is evident year round, with weakly and strongly absorbing biomass particles dominant in the autumn and winter months, respectively, while particles exhibit variable absorption during the spring season. A classification method using &alpha;_{440&ndash;870} and &omega;_oabs440 is developed in order to infer the seasonal physico-chemical properties of the aerosol types, such as fine and coarse mode, weak and strong absorption, at the four selected Asian sites

[1] Asian dust events occur frequently during the boreal spring season. Their optical properties have been analyzed by using a combination of source region (ground-based and satellite) and remote Pacific Ocean (aircraft) measurements during the Intercontinental Chemical Transport Experiment-Phase B (INTEX-B) field campaign which lasted from 7 April to 15 May 2006. A strong dust event originating from the Gobi Desert and passing over the Xianghe surface site on 17 April 2006 has been extensively analyzed. The surface averaged aerosol optical depth (AOD) values increased from 0.17 (clear sky) to 4.0 (strong dust), and the Angström exponent (a) dropped from 1.26 (clear sky) to below 0.1. Its total downwelling SW flux over the Xianghe site (thousands of kilometers away from the dust source region) is only 46% of the clear-sky value with almost no direct transmission and nearly double the diffuse SW clear-sky value. This event was also captured 6 days later by satellite observations as well as the UND/NASA DC-8 aircraft over the eastern Pacific Ocean. The DC-8 measurements in the remote Pacific region further classified the plumes into dust dominant, pollution dominant, and a mixture of dust and pollution events. HYSPLIT backward trajectories not only verified the origins of each case we selected but also showed (1) two possible origins for the dust: the Gobi and Taklimakan deserts; and (2) pollution: urban areas in eastern China, Japan, and other industrialized cities east of the two deserts. Based on the averaged satellite retrieved AOD data (0.5°× 0.5°grid box), declining AOD values with respect to longitude demonstrated the evolution of the transpacific transport pathway of Asian dust and pollution over the period of the field campaign.Citation: Logan, T., B. Xi, X. Dong, R. Obrecht, Z. Li, and M. Cribb (2010), A study of Asian dust plumes using satellite, surface, and aircraft measurements during the INTEX-B field experiment,

The radiative and microphysical properties of Saharan dust are believed to impact the Atlantic regional climate and tropical cyclones (TCs), but the detailed mechanism remains uncertain. In this study, atmosphere-only simulations are performed from 2002 to 2006 using the Community Atmospheric Model, version 5.1, with and without dust emission from the Sahara Desert. The Saharan dust exhibits noticeable impacts on the regional longwave and shortwave radiation, cloud formation, and the convective systems over West Africa and the tropical Atlantic. The African easterly jet and West African monsoon are modulated by dust, leading to northward shifts of the intertropical convergence zone and the TC genesis region. The dust events induce positive midlevel moisture and entropy deficit anomalies, enhancing the TC genesis. On the other hand, the increased vertical wind shear and decreased low-level vorticity and potential intensity by dust inhibit TC formation in the genesis region. The ventilation index shows a decrease in the intensification region and an increase in the genesis region by dust, corresponding to favorable and unfavorable TC activities, respectively. The comparison of nondust scenarios in 2005 and 2006 shows more favorable TC conditions in 2005 characterized by higher specific humidity and potential intensity, but lower ventilation index, wind shear, and entropy deficit. Those are attributable to the observed warmer sea surface temperature (SST) in 2005, in which dust effects can be embedded. Our results imply significant dust perturbations on the radiative budget, hydrological cycle, and large-scale environments relevant to TC activity over the Atlantic.