Recent progress in additive manufacturing (AM) allows for printing customized products with multiple materials and complex geometries that could form the basis of multimaterial designs with high performance and novel functions. Effectively designing such complex products for optimal performance within the confines of AM constraints is challenging due to the need to consider fabrication constraints while searching for optimal designs with a large number of variables, which stem from new AM capabilities. In this study, fabrication constraints are addressed through empirically characterizing multiple printed materials' Young's modulus and density using a multimaterial inkjet-based 3D-printer. Data curves are modeled for the empirical data describing two base printing materials and 12 mixtures of them as inputs for a computational optimization process. An optimality criteria (OC) method is developed to search for solutions of multimaterial lattices with fixed topology and truss cross section sizes. Two representative optimization studies are presented and demonstrate higher performance with multimaterial approaches in comparison to using a single material. These include the optimization of a cubic lattice structure that must adhere to a fixed displacement constraint and a compliant beam lattice structure that must meet multiple fixed displacement constraints. Results demonstrate the feasibility of the approach as a general synthesis and optimization method for multimaterial, lightweight lattice structures that are large-scale and manufacturable on a commercial AM printer directly from the design optimization results.

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The properties of periodic cellular structures strongly depend on the regular spatial arrangement of their constituent base materials and can be controlled by changing the topology and geometry of the repeating unit cell. Recent advances in three-dimensional (3D) fabrication technologies more and more expand the limits of fabricable real-world architected materials and strengthen the need of novel microstructural topologies for applications across all length scales and fields in both fundamental science and engineering practice. Here, we systematically explore, interpret, and analyze publicly available crystallographic network topologies from a structural point of view and provide a ready-to-use unit cell catalog with more than 17,000 unique entries in total. We show that molecular crystal networks with atoms connected by chemical bonds can be interpreted as cellular structures with nodes connected by mechanical bars. By this, we identify new structures with extremal properties as well as known structures such as the octet-truss or the Kelvin cell and show how crystallographic symmetries are related to the mechanical properties of the structures. Our work provides inspiration for the discovery of novel cellular structures and paves the way for computational methods to explore and design microstructures with unprecedented properties, bridging the gap between microscopic crystal chemistry and macroscopic structural engineering.