Considering the disadvantages of the common methods for CsPbBr 3 single crystal growth including the high cost of the melt method and the low shape controllability of the solution method, a facile hot-pressed (HP) approach has been introduced to prepare CsPbBr 3 wafers. The effects of HP temperature on the phase purity of HP-CsPbBr 3 wafers and the performance of the corresponding photodetectors have been investigated. The HP temperature for preparing phase-pure, shape-regular, and dense CsPbBr 3 wafers has been optimized to be 150 °C, and the HP-CsPbBr 3 wafer based planar-type photodetectors exhibit an ultrasensitive weak light photoresponse. Under the illumination of a 530 nm LED with a light power density of 1.1 μW cm −2 , the responsivity, external quantum efficiency, and detectivity of the devices reach 19.79 A W −1 , 4634%, and 2.14 × 10 13 Jones, respectively, and a fast response speed with a rise time of 40.5 μs and a fall time of 10.0 μs has been achieved.
Carbon nanotubes (CNTs) are ultimately small structures, attractive for future nanoelectronics. CNT-bundles on Si nanostructures can offer an alternative pathway to build hybrid CMOS-compatible devices. To develop a simple method of using such CNT-bundles as transistor channels, we fabricated semiconductor single-walled CNT field-effect transistors using inkjet printing on a CMOS-compatible platform. We investigated a method of producing stable CNT solutions without surfactants, allowing for CNT debundling and dispersion. An inkjet-printing system disperses CNT-networks with ultimately low density (down to discrete CNT-bundles) in Al source-drain gaps of transistors. Despite the small number of networks and random positions, such CNT-bundles provide paths to the flow current. For enhanced controllability, we also demonstrate the manipulation of CNT-networks using an AFM technique.
A series of LaF3:Ce3+ phosphors for application in photodynamic therapy are synthesized using a one-stage solvothermal synthesis. The synthesis conditions; type and quantity of stabilizer; concentration of activator providing the maximum intensity of UV- and X-ray-excited luminescence; lowest size; and highest colloidal stability of the phosphor nanoparticles are found. As a result of this study, the following parameters are determined using cerium content 5% mol. ethanol as the reaction medium for the solvothermal synthesis and polyvinylpyrrolidone as the stabilizer at an optimized amount.
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