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Fluctuating plume models provide a useful conceptual paradigm in the understanding of plume dispersion in a turbulent flow. In particular, these models have enabled analytical predictions of higher-order concentration moments, and the form of the one-point concentration probability density function (PDF). In this paper, we extend the traditional formalism of these models, grounded in the theory of homogeneous and isotropic turbulent flow, to two cases: namely, a simple sheared boundary layer and a large array of regular obstacles. Some very high-resolution measurements of plume dispersion in a water channel, obtained using laser-induced fluorescence (LIF) line-scan techniques are utilised. These data enable us to extract time series of plume centroid position (plume meander) and dispersion in the relative frame of reference in unprecedented detail. Consequently, experimentally extracted PDFs are able to be directly compared with various theoretical forms proposed in the literature. This includes the PDF of plume centroid motion, the PDF of concentration in the relative frame, and a variety of concentration moments in the absolute and relative frames of reference. The analysis confirms the accuracy of some previously proposed functional forms of model components used in fluctuating plume models, as well as suggesting some new forms necessary to deal with the complex boundary conditions in the spatial domain.

We report on measurements of the near-field dispersion of contaminant plumes in a large array of building-like obstacles at three scales; namely, at fullscale in a field experiment, at 1:50 scale in a wind-tunnel simulation, and at 1:205 scale in a water-channel simulation. Plume concentration statistics extracted from the physical modelling in the wind-tunnel and water-channel simulations are compared to those obtained from a field experiment. The modification of the detailed structure of the plume as it interacts with the obstacles is investigated. To this purpose, measurements of the evolution of the mean concentration, concentration fluctuation intensity, concentration probability density function, and integral time scale of concentration fluctuations in the array plume obtained from the field experiment and the scaled wind-tunnel and water-channel experiments are reported and compared, as well as measurements of upwind and within-array velocity spectra. Generally, the wind-tunnel and water-channel results on the modification of the detailed plume structure by the obstacles were qualitatively similar to those observed in the field experiments. However, with the appropriate scaling, the water-channel simulations were able to reproduce quantitatively the results of the full-scale field experiments better than the wind-tunnel simulations.

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