In the research area of strong-laser-field interactions and attosecond science 1 , tunnelling of an electron through the barrier formed by the electric field of the laser and the atomic potential is typically assumed to be the initial key process that triggers subsequent dynamics [1][2][3] . Here we use the attoclock technique 4 to obtain experimental information about the electron tunnelling geometry (the natural coordinates of the tunnelling current flow) and exit point. We confirm vanishing tunnelling delay time, show the importance of the inclusion of Stark shifts 5,6 and report on multi-electron effects clearly identified by comparing results in argon and helium atoms. Our combined theory and experiment allows us to single out the geometry of the inherently one-dimensional tunnelling problem, through an asymptotic separation of the full three-dimensional problem. Our findings have implications for laser tunnel ionization in all atoms and in particular in larger molecular systems with correspondingly larger dipoles and polarizabilities.One of the most striking manifestations of the rules of quantum mechanics is the possibility for a particle to move from one side of a potential barrier to the other regardless of the energy height of that barrier. This includes the classically forbidden case, referred to as tunnelling, where the potential energy of the barrier is higher than the energy of the particle (Fig. 1a). In linearly polarized laser fields, electron tunnelling is expected to eventually lead to above-threshold ionization, enhanced double ionization and coherent emission up to the X-ray regime with high-order harmonic generation [7][8][9][10] . Therefore, a detailed understanding of the tunnelling step is of paramount importance for attosecond science, including generation of attosecond pulses 11,12 and attosecond measurement techniques 4,13,14 . The attoclock 4 is an attosecond streaking technique 13 . The rotating electric field vector of a close-to-circularly polarized laser field gives the time reference, in a manner similar to the hands of a clock, and the time is measured by counting fractions of cycles with the exact angular position of the rotating electric field. In this way it is possible to obtain attosecond time resolution by employing a femtosecond pulse. The attoclock was used to set an upper limit to the tunnelling delay time during the tunnel ionization process in helium 15 , and to measure the ionization times in double ionization of argon 16,17 . For the attoclock, a very short few-femtosecond pulse is used to both ionize an atom and to provide the time reference. The pulse duration is kept sufficiently short such that the ionization event is limited to within one optical cycle around the peak of the pulse. As a result of the close-to-circular polarization, re-scattering of the liberated electron with the parent ion is mostly suppressed. Assuming classical 1 Physics Department, ETH Zurich, 8093 Zurich, Switzerland, 2 Lundbeck Foundation Theoretical Center for Quantum System Research, De...
We investigate the differences in the dynamics of lasers mode-locked by fast and slow saturable absorbers. Slow saturable absorbers can already generate almost transform limited pulses much shorter than the recovery time of the absorber. If soliton-like pulse shaping is present in addition the pulses can be further compressed below the resulting net gain window until either the continuum breaks through or the pulses break up into multiple pulses, which sets a limit to the shortest pulsewidth achievable. Given a certain amount of saturable absorption, a comparison is made that results in an estimate for the shortest pulse achievable for a solitary laser stabilized by a fast or a slow saturable absorber. The theoretical results are compared with experiments.
We show that a soliton of the nonlinear Schrödinger equation perturbed by filter losses and/or the finite gain bandwidth of amplifiers can be kept stable by saturable absorbers with a relaxation time much longer than the width of the soliton. This provides for ultrashort pulse generation with a slow saturable absorber only and may have possible applications in the stabilization of soliton storage rings.
We present a semiconductor saturable absorber mirror mode-locked thin disk laser based on Yb:Lu(2)O(3) with an average power of 141 W and an optical-to-optical efficiency of more than 40%. The ideal soliton pulses have an FWHM duration of 738 fs, an energy of 2.4 microJ, and a corresponding peak power of 2.8 MW. The repetition rate was 60 MHz and the beam was close to the diffraction limit with a measured M(2) below 1.2.
We demonstrate a power-scalable concept for high-power all-solid-state femtosecond lasers, based on passive mode locking of Yb:YAG thin disk lasers with semiconductor saturable-absorber mirrors. We obtained 16.2 W of average output power in pulses with 730-fs duration, 0.47-muJ pulse energy, and 560-kW peak power. This is to our knowledge the highest average power reported for a laser oscillator in the subpicosecond regime. Single-pass frequency doubling through a 5-mm-long lithium triborate crystal (LBO) yields 8-W average output power of 515-nm radiation.
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