Spin-polarized scanning tunneling microscopy (SP-STM) has been used extensively to study magnetic properties of nanostructures. Using SP-STM to visualize magnetic order in strongly correlated materials on an atomic scale is highly desirable, but challenging. We achieved this goal in iron tellurium (Fe(1+ y)Te), the nonsuperconducting parent compound of the iron chalcogenides, by using a STM tip with a magnetic cluster at its apex. Our images of the magnetic structure reveal that the magnetic order in the monoclinic phase is a unidirectional stripe order; in the orthorhombic phase at higher excess iron concentration (y > 0.12), a transition to a phase with coexisting magnetic orders in both directions is observed. It may be possible to generalize the technique to other high-temperature superconductor families, such as the cuprates.
Establishing the relation between ubiquitous antiferromagnetism in the parent compounds of unconventional superconductors and their superconducting phase is important for understanding the complex physics in these materials. Going from bulk systems to thin films additionally affects their phase diagram. For Fe1+yTe, the parent compound of Fe1+ySe1−xTex superconductors, bulk-sensitive neutron diffraction revealed an in-plane oriented diagonal double-stripe antiferromagnetic spin structure. Here we show by spin-resolved scanning tunnelling microscopy that the spin direction at the surfaces of bulk Fe1+yTe and thin films grown on the topological insulator Bi2Te3 is canted out of the high-symmetry directions of the surface unit cell resulting in a perpendicular spin component, keeping the diagonal double-stripe order. As the magnetism of the Fe d-orbitals is intertwined with the superconducting pairing in Fe-based materials, our results imply that the superconducting properties at the surface of the related superconducting compounds might be different from the bulk.
Articles you may be interested in Design of a scanning gate microscope for mesoscopic electron systems in a cryogen-free dilution refrigerator Rev. Sci. Instrum. 84, 033703 (2013); 10.1063/1.4794767 Construction and performance of a dilution-refrigerator based spectroscopic-imaging scanning tunneling microscope Rev. We develop a small-signal measurement system on cryogen-free dilution refrigerator which is suitable for superconducting qubit studies. Cryogen-free refrigerators have several advantages such as less manpower for system operation and large sample space for experiment, but concern remains about whether the noise introduced by the coldhead can be made sufficiently low. In this work, we demonstrate some effective approaches of acoustic isolation to reduce the noise impact. The electronic circuit that includes the current, voltage, and microwave lines for qubit coherent state measurement is described. For the current and voltage lines designed to have a low pass of dc-100 kHz, we show that the measurements of Josephson junction's switching current distribution with a width down to 1 nA, and quantum coherent Rabi oscillation and Ramsey interference of the superconducting qubit can be successfully performed.
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