The management of spontaneous light emission at the nanoscale is a crucial aspect in many application domains dealing with lighting, optical communications and quantum information systems. Two widespread approaches to target this topic are based on plasmonic structures and dielectric photonic crystals, which have demonstrated a high potential in controlling spectral, angular and temporal features of the emission. Both approaches exhibit rather complementary advantages, and many efforts are nowadays undertaken to find hybrid solutions taking the best from the two sides.In his framework, we propose a photonic device based on a dielectric multilayer, which is shown to control the spontaneous emission from organic dyes embedded therein. Such a result is achieved by exploiting the near-field interaction of emitters to Bloch Surface Waves resonantly coupled within a sub-wavelength cavity surrounded by a diffractive structure. A bright, monochromatic spontaneous emission is then obtained, with spectral width below 1 nm, a decay rate increased by a factor spanning from 16 to 33, and a propagation divergence below 5 degrees in free space. These findings are particularly promising for application in integrated photonic circuits and single-photon sources.
Metal nanostructures (such as plasmonic antennas) have been widely demonstrated to be excellent devices for beaming and sorting the fluorescence emission. These effects rely on the constructive scattering or diffraction from different elements (such as metal corrugations or nanorings) of the nanostructures. However, subwavelength-size nanoholes, without nearby nanoscale features, results in an angularly dispersed emission from the distal surface. Herein, we demonstrate for the first time the emission redirection capabilities of a single isolated nanoaperture milled in a thick silver film deposited on a dielectric multilayer. Specifically, we show that a dye dissolved in ethanol filling in the nanoaperture can couple to Tamm Plasmon Polariton (TPP) modes of the structure. Due to the small in-plane wavevectors of the TPPs, the fluorescence from Tamm-coupled dyes within the nanoaperture is emitted normally to the sample surface, with a minimum angular width of about 12.54°. This kind of fluorescence manipulation has proven to be effective with various nanoaperture shapes, such as circles, squares, and triangles. Our work is also the first experimental demonstration of lateral coupling of fluorophores with TPPs in nanoholes, with potential applications in bioanalysis and biosciences.
Axis-symmetric grooves milled in metallic slabs have been demonstrated to promote the transfer of Orbital Angular Momentum (OAM) from far- to near-field and vice versa, thanks to spin-orbit coupling effects involving Surface Plasmons (SP). However, the high absorption losses and the polarization constraints, which are intrinsic in plasmonic structures, limit their effectiveness for applications in the visible spectrum, particularly if emitters located in close proximity to the metallic surface are concerned. Here, an alternative mechanism for vortex beam generation is presented, wherein a free-space radiation possessing OAM is obtained by diffraction of Bloch Surface Waves (BSWs) on a dielectric multilayer. A circularly polarized laser beam is tightly focused on the multilayer surface by means of an immersion optics, such that TE-polarized BSWs are launched radially from the focused spot. While propagating on the multilayer surface, BSWs exhibit a spiral-like wavefront due to the Spin-Orbit Interaction (SOI). A spiral grating surrounding the illumination area provides for the BSW diffraction out-of-plane and imparts an additional azimuthal geometric phase distribution defined by the topological charge of the spiral structure. At infinity, the constructive interference results into free-space beams with defined combinations of polarization and OAM satisfying the conservation of the Total Angular Momentum, based on the incident polarization handedness and the spiral grating topological charge. As an extension of this concept, chiral diffractive structures for BSWs can be used in combination with surface cavities hosting light sources therein.
Multispectral plasmonic color filters were fabricated using nano-imprint lithography and benchmarked to similar filters fabricated with standard CMOS processing. The self-aligned process yields devices with narrow linewidths below 30nm and up to 50% transmission efficiency.
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