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Several diverse types of UH 3 -based hydrides can be prepared by hydrogenation of bcc Ubased alloys. Pair Distribution Function (PDF) analysis using high-energy X-rays identified that the (UH 3 ) 1-x Mo x hydrides are nanocrystalline, with the structure motif based mainly on the -UH 3 structure. -UH 3 represents a minority component. On the other hand, PDF of the (UH 3 ) 1-x Zr x hydrides corresponds well to the -UH 3 crystal structure. All the hydrides are ferromagnetic, with the Curie temperature T C reaching up to 203 K.

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