The measurement of photon-number statistics of fields composed of photon pairs, generated in spontaneous parametric down-conversion and detected by an intensified charge-coupled device (iCCD) camera, is described. Final quantum detection efficiencies, electronic noises, finite numbers of detector pixels, transverse intensity spatial profiles of the detected beams, as well as losses of single photons from a pair are taken into account in a developed general theory of photon-number detection. The measured data provided by an iCCD camera with single-photon detection sensitivity are analyzed along the developed theory. Joint signal-idler photon-number distributions are recovered using the reconstruction method based on the principle of maximum likelihood. The range of applicability of the method is discussed. The reconstructed joint signal-idler photon-number distribution is compared with that obtained by a method that uses superposition of signal and noise and minimizes photoelectron entropy. Statistics of the reconstructed fields are identified to be multimode Gaussian. Elements of the measured as well as the reconstructed joint signal-idler photon-number distributions violate classical inequalities. Sub-shot-noise correlations in the difference of the signal and idler photon numbers as well as partial suppression of odd elements in the distribution of the sum of signal and idler photon numbers are observed.
In this paper, we establish connections between the thresholds and mechanisms of the damage and white-light generation upon femtosecond laser irradiation of wide-bandgap transparent materials. On the example of Corning Willow glass, evolution of ablation craters, their quality, and white-light emission were studied experimentally for 130-fs, 800-nm laser pulses. The experimental results indicate co-existence of several ablation mechanisms which can be separated in time. Suppression of the phase explosion mechanism of ablation was revealed at the middle of the irradiation spots. At high laser fluences, air ionization was found to strongly influence ablation rate and quality and the main mechanisms of the influence are analysed. To gain insight into the processes triggered by laser radiation in glass, numerical simulations have been performed with accounting for the balance of laser energy absorption and its distribution/redistribution in the sample, including bremsstrahlung emission from excited free-electron plasma. The simulations have shown an insignificant role of avalanche ionization at such short durations of laser pulses while pointing to high average energy of electrons up to several dozens of eV. At multi-pulse ablation regimes, improvement of crater quality was found as compared to single/few pulses.
Coherence properties of the down-converted beams generated in spontaneous parametric down-conversion are investigated in detail using an iCCD camera. Experimental results are compared with those from a theoretical model developed for pulsed pumping with a Gaussian transverse profile. The results allow us to tailor the shape of correlation area of the signal and idler photons using pump-field and crystal parameters. As an example, splitting of a correlation area caused by a two-peak pump-field spectrum is experimentally studied.
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