The present work is dedicated to study of the possibilities of improving the production method of 11 C and 18 F medical isotopes using a linear electron accelerator. Experimental studies of 11 C and 18 F isotopes production by the photonuclear technique were carried out in [1]. Various targets were irradiated by bremsstrahlung photons following by measurements targets' activities. This experimental research has been carried out in the energy range from 10 to 40 MeV. The current work studies an angular distribution of bremsstrahlung photons in order to estimate the possibilities of producing maximum achievable levels of medical isotopes 18 F and 11 С activities. The angular distribution of bremsstrahlung photons is an important property of the irradiation stand which contains an assembly of targets. This important property allows designing necessary changes in the target assembly setup used to produce medical isotopes. The research presented in the current work was done as a computer simulation. The computer software package 'KIPT' was developed in С++ programming language, using the Geant4 toolkit in order to obtain the angular distribution of bremsstrahlung photons. Experimental setup materials as well as structural elements positions were defined in the DetectorConstruction class of our program. The parameters of an electron beam were defined in the PrimaryGeneratorAction class. The electron beam diameter was defined as 8 mm, energy Е е =36.7 MeV, corresponding to the real experiment carried out at the "Accelerator" Science and Research Establishment of Kharkiv Institute of Physics and Technology [1]. Models of physical processes occurring while the electron beam crosses the target assembly were defined in the PhysicsList class. All classes and modules necessary for the analysis of simulation results were included to our program together with visualization modules. Visualization modules use the OpenGL graphics library and the Qt5 software to represent the relative position of experimental setup parts and to visualize particle trajectories. As a result of this work, the angular distributions were obtained for the beam of electrons and bremsstrahlung photons directly before the target. This result will allow target assembly parameter optimization for optimal production of medical isotopes by the photonuclear technique.
The proposed work demonstrates the results of creating and investigating the mathematical model of the source of fast neutrons. Computer modeling of the energy spectrum of fast neutrons was carried out for 239PuBe neutron source. The model of the source of fast neutrons has been developed. Neutrons in this model have an energy spectrum from 100 keV to 11 MeV with 100 keV step. Simulation is performed by the Monte-Carlo method. The model carrier is a computer program developed in the C++ programming language in the Linux operating system environment, using the Geant4 toolkit. All necessary classes describing low-energy models were used for the simulation of the passage of neutrons through materials of detectors. Those take into account the elastic scattering, inelastic scattering, radiative capture and fission. We consider these processes because models of processes implemented in our software will be also used for other problems of neutrons transport, for example, for passing neutrons through various substances, and for conducting virtual laboratory works. The PhysicsList class of our program contains classes G4NeutronHPElastic, G4NeutronHPElasticData, G4NeutronHPInelastic, G4NeutronHPInelasticData, G4NeutronHPCapture, G4NeutronHPCaptureData, etc. based on the NeutronHP model for neutron interactions at low energy, as well as the neutron data library G4NDL4.5. Diagrams containing energy spectra of a source of fast neutrons modeled in two ways are presented in the paper. The analysis of the obtained energy spectra is carried out. Virtual nuclear physics experiments are carried out with the aim of testing the elaborated neutron-matter interaction model. The processes occurring in scintillator substances during the passage of fast neutrons through them, have been studied. 109 neutrons were used as primary particles emitted isotropically, and we used our simulation results of 239PuBe neutron source to describe the initial energy spectrum. The created model of 239PuBe neutron source can be used for the investigation of scintillation detectors Bi4Ge3O12, CdWO4, Gd2SiO5 and others, as well as studying their characteristics. Processes in heavy oxide scintillators substance during the registration of fast neutrons can be studied using the developed model. It is shown that for registration of the flow of neutrons from 239PuBe neutron source, using Bi4Ge3O12 or CdWO4 scintillators is more preferable. Results of the virtual nuclear physical experiments satisfy the published experimental data.
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