We study the problem of magnetization and heat currents and their associated thermodynamic forces in a magnetic system by focusing on the magnetization transport in ferromagnetic insulators like YIG. The resulting theory is applied to the longitudinal spin Seebeck and spin Peltier effects. By focusing on the specific geometry with one Y3Fe5O12 (YIG) layer and one Pt layer, we obtain the optimal conditions for generating large magnetization currents into Pt or large temperature effects in YIG. The theoretical predictions are compared with experiments from the literature permitting to derive the values of the thermomagnetic coefficients of YIG: the magnetization diffusion length lM ∼0.4 μm and the absolute thermomagnetic power coefficient εM∼10−2 TK−1
In this paper we present the results of an experimental investigation of the magnetocaloric properties of hydrogenated La(Fe-Mn-Si) 13 -H with Mn substituting Fe to finely tune the transition temperature. We measured the specific heat under magnetic field c p (H, T ) and the magnetic field induced isothermal entropy change ∆s(H, T ) of a series of compounds by direct Peltier calorimetry. Results show that increasing Mn from 0.06 to 0.46 reduces the transition temperature from 339 K to 270 K whilst the total entropy change due to a 1.5 T field is depressed from 18.7 Jkg −1 K −1 to 10.2 Jkg −1 K −1 and the thermal hysteresis similarly is reduced from 1.5 K to zero. In the paper we interpret the results in terms of a magnetic phase transition changing from the first to the second order with increasing Mn content and we discuss the value of the results for magnetic cooling applications.
The determination of the longitudinal spin Seebeck effect (LSSE) coefficient is currently plagued by a large uncertainty due to the poor reproducibility of the experimental conditions used in its measurement. In this work we present a detailed analysis of two different methods used for the determination of the LSSE coefficient. We have performed LSSE experiments in different laboratories, by using different setups and employing both the temperature difference method and the heat flux method. We found that the lack of reproducibility can be mainly attributed to the thermal contact resistance between the sample and the thermal baths which generate the temperature gradient. Due to the variation of the thermal resistance, we found that the scaling of the LSSE voltage to the heat flux through the sample rather than to the temperature difference across the sample greatly reduces the uncertainty. The characteristics of a single YIG/Pt LSSE device obtained with two different setups was (1.143 ± 0.007) 10−7 Vm/W and (1.101 ± 0.015) 10−7 Vm/W with the heat flux method and (2.313 ± 0.017) 10−7 V/K and (4.956 ± 0.005) 10−7 V/K with the temperature difference method. This shows that systematic errors can be considerably reduced with the heat flux method.
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