New experimental and theoretical results for the material parameter reconstruction using terahertz (THz) pulsed spectroscopy (TPS) are presented. The material parameter reconstruction algorithm was realized and experimentally implemented to study the test sample. In order to both verify the algorithm and to estimate the reconstruction accuracy, test sample material parameters obtained with the TPS were compared with the results of the same sample studying by the use of the backward-wave oscillator (BWO) spectroscopy. Thus, high reconstruction accuracy was demonstrated for the spectral range, corresponding to the BWO sensitivity and located between 0.2 and 1.2 THz. The numerical simulations were applied for determining the material parameter reconstruction stability in the presence of white Gaussian noise in TPS waveforms as well as fluctuations in the femtosecond (FS) optical pulse duration. We report a strong dependence of the inverse problem solution stability on these factors. We found that the instability of the FS optical pulse duration used for THz pulses generation and detection limits the material parameter reconstruction with TPS.

Mid‐infrared materials antireflection is in high demand for high‐powered or ultra‐broadband coherent light sources, where conventional antireflection coatings cannot be reliably applied. This work provides a critical review of the recent advances in microstructure fabrication technology for mid‐infrared antireflection applications. Several techniques are reviewed, including direct imprinting, wet and reactive ion etching using conventional photoresist masking, novel colloid crystal masks, and maskless etching, laser‐induced periodic structure formation, and multiple laser ablation method modifications, including femtosecond laser direct writing, direct laser interference ablation, and single pulse ablation. The advantages and drawbacks of the different approaches are discussed in detail to highlight the most promising techniques for the fabrication of antireflection microstructures capable of achieving 99% transmittance in the 2–16 μm range.

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We report a study on the switching of the generation regimes in a high-powered thulium-doped all-fiber ring oscillator that is passively mode-locked with nonlinear polarization evolution technique with different pumping rates and cavity dispersion values. In one experimental setup, switching was observed between the noise-like pulse and the multi-soliton (in the forms of soliton bunches and soliton rain) regimes by the adjustment of the intracavity polarization controllers. We attributed this to the crucial influence of the nonlinear polarization evolution strength determined by such key parameters as saturation (over-rotation) power, linear phase bias, and nonlinear losses on the pulse evolution and stability. So the soliton collapse effect (leading to noise-like pulse generation) or the peak power clamping effect (generating a bunch of loosely-bound solitons) may determine pulse dynamics. Both the spectrum bandwidth and coherence time were studied for noise-like pulses by varying the cavity length and pump power, as well as the duration of solitons composing bunches. As a result, both noise-like pulses (with spectrum as broad as 32 nm bandwidth) and multi-soliton formations (with individual pulse-widths ranging from 748 to 1273 fs with a cavity length increase from 12 to 53 m) with up to 730 mW average power were generated at a wavelength of around 1.9 μm. The results are important for the realization of the broadband and smooth supercontinuum which can be used as a source for mid-IR vibrational spectroscopy of gas samples for breath analysis and environmental sensing.

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