A ferromagnet/antiferromagnet (FM/AFM) Fe/NiO bilayer was grown using molecular beam epitaxy on MgO(001) and Cr buffered MgO(001) substrates. X-ray linear dichroism measurements showed a dominating out-of-plane component for the NiO spins in Fe/NiO/MgO and an in-plane spin direction for NiO layers grown on the Cr buffer. Furthermore, systematic studies on the magnetic properties of Fe/NiO grown on the wedge-shaped Cr buffer revealed a continuous strain-induced spin reorientation transition from out-of-plane to in-plane NiO spin directions when the Cr thickness increased from 0 nm to 3.5 nm. The analysis of the in-plane magnetic structure of NiO in Fe/NiO/Cr showed a pronounced uniaxial anisotropy in thin AFM layers. The AFM spins are perpendicular to the Fe spins due to spin–flop interaction. These results demonstrate the feasibility of using strain and coupling with FMs to manipulate spin structures in NiO.

We show that in a uniform thickness NiO(111)/Fe(110) epitaxial bilayer system, at given temperature near 300 K, two magnetic states with orthogonal spin orientations can be stabilized in antiferromagnetic NiO.

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In our study, we examined the chemical and magnetic properties of FeO in an epitaxial Fe/MgO(dMgO)/FeO trilayer for different MgO thicknesses, dMgO. Analysis of the chemical structure revealed a stoichiometry improvement in the FeO layer in Fe/MgO/FeO in comparison with a Fe/FeO bilayer. Furthermore, we showed that deposition of a subtle MgO layer at the Fe/FeO interface results in an enhanced exchange interaction between Fe and FeO. For dMgO = 1.4 Å, we noted a 200% enhancement in the exchange bias in Fe/MgO/FeO compared to that in Fe/FeO.