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Effective soil erosion prediction models and proper conservation practices are important tools to mitigate soil erosion in hillside agricultural areas. The Water Nutrient and Light Capture in Agroforestry Systems (WaNuLCAS) and Water Erosion Prediction Project (WEPP) models are capable tools in soil erosion simulation in the conventional and conservation cropping systems in hillslopes. We calibrated both the models in maize monocropping and simultaneously validated them in maize-chili intercropping with Leucaena hedgerow for nine rainfall events in 2010, with the aim to evaluate their performances in runoff and sediment prediction on a skeleton soil in a hillslope, Western Thailand. The results showed that the calibrated WaNuLCAS model poorly predicts runoff prediction in the validation. In contrast, the calibrated WEPP model had a better performance in runoff prediction in the validation. For sediment prediction, the calibrated WaNuLCAS model predicted sediment yield better than the calibrated WEPP model in the validation because the WEPP model shows more variability of the sediment yield in the calibration (5.84 kg m –2 ) than the WaNuLCAS (5.18 kg m –2 ). Thus, the WEPP model was more suitable for runoff prediction than sediment prediction in the monocropping system, whereas the WaNuLCAS model was better suited for sediment yield prediction than runoff prediction, especially in complex intercropping systems.