The vortex, a fundamental topological excitation featuring the in-plane winding of a vector field, is important in various areas such as fluid dynamics, liquid crystals, and superconductors. Although commonly existing in nature, vortices were observed exclusively in real space. Here, we experimentally observed momentum-space vortices as the winding of far-field polarization vectors in the first Brillouin zone of periodic plasmonic structures. Using homemade polarization-resolved momentum-space imaging spectroscopy, we mapped out the dispersion, lifetime, and polarization of all radiative states at the visible wavelengths. The momentum-space vortices were experimentally identified by their winding patterns in the polarization-resolved isofrequency contours and their diverging radiative quality factors. Such polarization vortices can exist robustly on any periodic systems of vectorial fields, while they are not captured by the existing topological band theory developed for scalar fields. Our work provides a new way for designing high-Q plasmonic resonances, generating vector beams, and studying topological photonics in the momentum space.
Bound states in the continuum in periodic photonic systems like photonic crystal slabs are proved to be accompanied by vortex polarization singularities on the photonic bands in the momentum space. The winding structures of polarization states not only widen the field of topological physics but also show great potential that such systems could be applied in polarization manipulating. In this work, we report the phenomenon that by in-plane inversion (C2) symmetry breaking, pairs of circularly polarized states could spawn from the eliminated Bound states in the continuum. Along with the appearance of the circularly polarized states as the two poles of the Poincaré sphere together with linearly polarized states covering the equator, full coverage on the Poincaré sphere could be realized. As an application, ellipticity modulation of linear polarization is demonstrated in the visible frequency range. This phenomenon provides new degree of freedom in modulating polarization.
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