After electrons tunnel out of a laser-Coulomb-formed barrier, the movement of the tunneling electron can be affected by the Coulomb potential. We show that this Coulomb effect induces a large time difference (longer than a hundred attoseconds) between the tunneling-out time at which the electron exits the barrier and the ionization time at which the electron is free. This large time difference has important influences on strong-field processes such as above-threshold ionization and high-harmonic generation, with remarkably changing time-frequency properties of electron trajectories. Some semi-quantitative evaluations on these influences are addressed, which provide new insight into strong-field processes and give suggestions on attosecond measurements.
We study odd-even high-harmonic generation (HHG) from oriented asymmetric molecules with different symmetries in strong laser fields. A model based on strong-field approximations is used which allows us to resolve the contributions of different emission routes to odd-even HHG. The comparison between the HHG yields of all routes versus one certain route demonstrates that the routes in which the electron ionizes from the gerade component of the asymmetric orbital contribute mainly to odd-even HHG. We show that the potential mechanism is associated with effects of intramolecular interference in tunneling ionization as the bound electron passes through the barrier formed by the laser field and the asymmetric Coulomb potential. The influences of different emission routes on asymmetric orbital imagining with odd-even HHG are also addressed.
We study the effect of Coulomb potential on high-order harmonic generation (HHG) numerically and analytically. We focus on the influence of Coulomb potential on emission times of HHG associated with specific electron trajectories. By using a numerical procedure based on numerical solution of time-dependent Schr\"{o}dinger equation (TDSE) in three dimensions, we extract the HHG emission times both for long and short electron trajectories. We compare TDSE predictions with those of a Coulomb-modified model arising from strong-field approximation (SFA). We show that the Coulomb effect induces earlier HHG emission times than those predicted by the general SFA model without considering the Coulomb potential. In particular, this effect influences differently on long and short electron trajectories and is more remarkable for low-energy harmonics than high ones. It also changes the HHG amplitudes for long and short electron trajectories. We validate our discussions with diverse laser parameters and forms of Coulomb potential. Our results strongly support a four-step model of HHG.
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