Org anic-inorganic halide perovskites have attracted considerable attention owing to their outstanding solar cell efficiency. Meanwhile, these halide perovskites exhibit good light emitting in visible and near-infrared range with high fluorescence quantum yield, resulting in electroluminescence. However, it remains challenging for lighting and display due to the low luminance and poor long-term stability. Herein, high performance green light-emitting diodes are fabricated from bromine based perovskite (CH3NH3PbBr3) by systematically adjusting the preparation conditions and optimizing the emitting layer thickness. A high luminance up to 1500 cd m −2 (one of the highest values for perovskites-based light-emitting diodes) was achieved with 80 nm perovskites-emitting layer, due to the well-crystallized, full-coverage property of the films. This result further confirms the great prospect of organic-inorganic perovskites in optoelectronics.Recently, organic-inorganic halide perov skites, a new class of semiconductors with high power conversion efficiency and long-range balanced hole-electron transport characteristics, have shown huge potential in photovoltaics [1−10]. However, the work principle of these perovskite materials has not been well elucidated except for a few reports [11−15]. Apart from charge mobility [16,17], optical properties clearly point out another way to investigate these materials, which show pieces of information including charge separation, bandgap and chemical purity [18]. Interestingly, these organic-inorganic materials based on perovskites really exhibit excellent photoluminescence properties with tunable visible and near-infrared spectru m [19−22]. Moreover, combined with their balanced ambipolar properties, these materials have been proven to be electrically light emission. Very recently, a breakthrough in light-emitting diodes (LEDs) based on organic-inorganic halide perovskites has been made, which proves organic-inorganic halide perovskites as promising candidates in LEDs [23]. The ever reported LEDs based on these halide perovskites which show electroluminescence in near-infrared, red and green region and a luminance of ~364 cd m −2 was achieved 1 B eijing National Laboratory for Molecular Sciences, Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China 2 University of Chinese Academy of Sciences, Beijing 100190, China * Corresponding authors (emails: dhl522@iccas.ac.cn (Dong H); huwp@iccas.ac.cn (Hu W)) when the thickness of the active layer was 20 nm. Lately, an improved luminance of 417 cd m −2 was obtained for multicolored perovskites-LEDs based on a 40 nm emitter layer, which is due to the reduced carrier injection barrier for efficient electroluminescence [24]. However, further application remains challenging owing to the toxicity of Pb atom, poor long-term stability and low luminance. Thus, improving the luminance, which is the focus of this paper, emerges as an important and urgent aspect to make these LEDs commercialized.Acco...
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.
customersupport@researchsolutions.com
10624 S. Eastern Ave., Ste. A-614
Henderson, NV 89052, USA
This site is protected by reCAPTCHA and the Google Privacy Policy and Terms of Service apply.
Copyright © 2024 scite LLC. All rights reserved.
Made with 💙 for researchers
Part of the Research Solutions Family.