In this Letter we experimentally demonstrate that the radiative heat transfer between metallic planar surfaces exceeds the blackbody limit by employing the near-field and thin-film effects. Nanosized polystyrene particles were used to create a nanometer gap between aluminum thin-films of different thicknesses coated on 5 × 5 mm 2 diced silicon chips while the gap spacing is fitted from the near-field measurement with bare Si chips. The experimental results are validated by theoretical calculation based on fluctuational electrodynamics. The near-field radiative heat flux between 13-nm Al thin-film samples at 215 nm gap distance is measured to be 6.4 times over the blackbody limit and 420 times compared to the far-field radiative heat transfer between metallic surfaces with a temperature difference of 65 K. In addition, the theoretical prediction suggests a near-field enhancement of 122 times relative to the blackbody limit and 8000 times over far-field one at 50-nm vacuum gap between 20-nm Al thin-film samples, under the same temperature difference of 65 K. This work will facilitate the understanding and application of near-field radiation to thermal power conversion, noncontact cooling, heat flow management, and optical storage where metallic materials are involved.
In this work we experimentally demonstrated the near-field thermal radiation enhancement over the blackbody limit by 11 times between highly doped silicon chips with 1×1 cm 2 size at a vacuum gap distance of 190±20 nm under a temperature difference of 74.7 K above room temperature. SU-8 polymer posts, which significantly reduced the conduction less than 6% of the total heat transfer due to its low thermal conductivity, were carefully fabricated with different heights to directly create vacuum gaps from 507±47 nm down to 190±20 nm precisely determined in-situ by capacitance measurement. Experimental results were validated by theoretical calculations based on fluctuational electrodynamics, which revealed the enhancement mechanism mainly as coupled surface plasmon polariton. The experimental method developed here will facilitate the potential applications of near-field radiative devices made of electrically conductive materials like metals, graphene, and transparent conductive oxide besides heavily doped semiconductors for thermal energy conversion, radiative thermal rectification, and radiative heat modulation.
We
experimentally demonstrate actively tunable infrared absorption
based on graphene-covered SiC metasurfaces. A dry transfer method
is employed to coat monolayer graphene on the metasurface characterized
by scanning electron microscope, atomic force microscopy, and Raman
spectroscopy. A solid polymer electrolyte is introduced to tune the
graphene chemical potential upon electrical gating. In situ optical measurement shows a shift in the absorption peak upon a
change in gate voltage. Numerical simulations unveil that the tuning
effect is attributed to the excitation of a magnetic polariton, whose
resonance frequency changes with graphene chemical potential upon
electrical gating. The reported results realize the possibility of
tuning thermal radiative property of a graphene-covered metasurface
through a solid polymer electrolyte, providing a new approach to fabricating
graphene-based tunable infrared devices for dynamic radiative thermal
management and sensing applications.
Summary
This work experimentally studies a silicon-cored tungsten nanowire selective metamaterial absorber to enhance solar-thermal energy harvesting. After conformally coating a thin tungsten layer about 40 nm thick, the metamaterial absorber exhibits almost the same total solar absorptance of 0.85 as the bare silicon nanowire stamp but with greatly reduced total emittance down to 0.18 for suppressing the infrared emission heat loss. The silicon-cored tungsten nanowire absorber achieves an experimental solar-thermal efficiency of 41% at 203°C during the laboratory-scale test with a stagnation temperature of 273°C under 6.3 suns. Without parasitic radiative losses from side and bottom surfaces, it is projected to reach 74% efficiency at the same temperature of 203°C with a stagnation temperature of 430°C for practical application, greatly outperforming the silicon nanowire and black absorbers. The results would facilitate the development of metamaterial selective absorbers at low cost for highly efficient solar-thermal energy systems.
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