Signaled by non-analyticities in the time evolution of physical observables, dynamic quantum phase transitions (DQPTs) emerge in quench dynamics of topological systems and possess an interesting geometric origin captured by dynamic topological order parameters (DTOPs). In this work, we report the experimental study of DQPTs using discrete-time quantum walks of single photons. We simulate quench dynamics between distinct Floquet topological phases using quantum-walk dynamics, and experimentally characterize DQPTs and the underlying DTOPs through interferencebased measurements. The versatile photonic quantum-walk platform further allows us to experimentally investigate DQPTs for mixed states and in parity-time-symmetric non-unitary dynamics for the first time. Our experiment directly confirms the relation between DQPTs and DTOPs in quench dynamics of a topological system, and opens up the avenue of simulating emergent topological phenomena using discrete-time quantum-walk dynamics.

We report the experimental detection of bulk topological invariants in nonunitary discrete-time quantum walks with single photons. The nonunitarity of the quantum dynamics is enforced by periodically performing partial measurements on the polarization of the walker photon, which effectively introduces loss to the dynamics. The topological invariant of the nonunitary quantum walk is manifested in the quantized average displacement of the walker, which is probed by monitoring the photon loss. We confirm the topological properties of the system by observing localized edge states at the boundary of regions with different topological invariants. We further demonstrate the robustness of both the topological properties and the measurement scheme of the topological invariants against disorder.

Topology in quench dynamics gives rise to intriguing dynamic topological phenomena, which are intimately connected to the topology of static Hamiltonians yet challenging to probe experimentally. Here we theoretically characterize and experimentally detect momentum-time skyrmions in parity-time -symmetric non-unitary quench dynamics in single-photon discrete-time quantum walks. The emergent skyrmion structures are protected by dynamic Chern numbers defined for the emergent two-dimensional momentum-time submanifolds, and are revealed through our experimental scheme enabling the construction of time-dependent non-Hermitian density matrices via direct measurements in position space. Our work experimentally reveals the interplay of symmetry and quench dynamics in inducing emergent topological structures, and highlights the application of discrete-time quantum walks for the study of dynamic topological phenomena.