The Kondo insulator SmB 6 has long been known to exhibit low temperature transport anomalies whose origin is of great interest. Here we uniquely access the surface electronic structure of the anomalous transport regime by combining state-of-the-art laser-and synchrotron-based angle-resolved photoemission techniques. We observe clear in-gap states (up to ∼ 4 meV), whose temperature dependence is contingent upon the Kondo gap formation. In addition, our observed in-gap Fermi surface oddness tied with the Kramers' points topology, their coexistence with the two-dimensional transport anomaly in the Kondo hybridization regime, as well as their robustness against thermal recycling, taken together, collectively provide by-far the strongest evidence for protected surface metallicity with a Fermi surface whose topology is consistent with the theoretically predicted topological surface Fermi surface. Our observations of systematic surface electronic structure provide the fundamental electronic parameters for the anomalous Kondo ground state of the correlated electron material SmB 6 .
In iron-pnictide superconductivity, the interband interaction between the hole and electron Fermi surfaces (FSs) is believed to play an important role. However, KFe(2)As(2) has three zone-centered hole FSs and no electron FS but still exhibits superconductivity. Our ultrahigh-resolution laser angle-resolved photoemission spectroscopy unveils that KFe(2)As(2) is a nodal s-wave superconductor with highly unusual FS-selective multi-gap structure: a nodeless gap on the inner FS, an unconventional gap with "octet-line nodes" on the middle FS, and an almost-zero gap on the outer FS. This gap structure may arise from the frustration between competing pairing interactions on the hole FSs causing the eightfold sign reversal. Our results suggest that the A(1g) superconducting symmetry is universal in iron-pnictides, in spite of the variety of gap functions.
Topological insulators and semimetals as well as unconventional iron-based superconductors have attracted major recent attention in condensed matter physics. Previously, however, little overlap has been identified between these two vibrant fields, even though the principal combination of topological bands and superconductivity promises exotic unprecedented avenues of superconducting states and Majorana bound states (MBSs), the central building block for topological quantum computation. Along with progressing laser-based spin-resolved and angle-resolved photoemission spectroscopy (ARPES) towards high energy and momentum resolution, we have resolved topological insulator (TI) and topological Dirac semimetal (TDS) bands near the Fermi level (E F ) in the iron-based superconductors Li(Fe,Co)As and Fe(Te,Se), respectively. The TI and TDS bands can be individually tuned to locate close to E F by carrier doping, allowing to potentially access a plethora of different superconducting topological states in the same material. Our results reveal the generic coexistence of superconductivity and multiple topological states in iron-based superconductors, rendering these materials a promising platform for high-T c topological superconductivity.High-T c iron-based superconductors feature multiple bands near E F , which enhances the difficulty in understanding the details of unconventional pairing 1-3 . It, however, also allows for a wealth of, possibly topologically non-trivial, electronic bands, of which a recent example is the TI states discovered in the ironbased superconductor Fe(Te,Se) 4 , hinting at a promising direction to realize topological superconductivity and MBSs 5-9 . In view of Fe(Te,Se), a pressing subsequent question is to which extent this marks a generic phe-nomenon in different classes of iron-based high-T c superconductors. In this work, we find that the emergence of non-trivial topological bands near the Fermi level is indeed a common feature of various iron-based superconductors. Our first-principles calculations reveal that BaFe 2 As 2 , LiFeAs and Fe(Te,Se) all exhibit band inversions along k z . To confirm these calculations, the band structures of Li(Fe,Co)As and Fe(Te,Se) were investigated by laser-based high-resolution ARPES. Firstly, we observe that TI bands reminiscent of Fe(Te,Se) exist in Li(Fe,Co)As as well, supporting the generic existence of non-trivial topology in iron-based superconductors. Secondly and more interestingly, we predict and observe TDS bands in Li(Fe,Co)As and Fe(Te,Se), which we investigate via high-resolution ARPES, spin-resolved ARPES (SARPES), and magnetoresistance (MR) measurements. Finally, we discuss the phase diagram of these topological high-T c compounds as a function of Fermi level (doping). The combination of topological states and superconductivity may produce not only surface topological superconductivity deriving from the TI edge states, but also bulk topological superconductivity from the TDS bands.Normal insulator (NI), TI, and TDS constitute topologically disti...
Strong spin–orbit coupling fosters exotic electronic states such as topological insulators and superconductors, but the combination of strong spin–orbit and strong electron–electron interactions is just beginning to be understood. Central to this emerging area are the 5d transition metal iridium oxides. Here, in the pyrochlore iridate Pr2Ir2O7, we identify a non-trivial state with a single-point Fermi node protected by cubic and time-reversal symmetries, using a combination of angle-resolved photoemission spectroscopy and first-principles calculations. Owing to its quadratic dispersion, the unique coincidence of four degenerate states at the Fermi energy, and strong Coulomb interactions, non-Fermi liquid behaviour is predicted, for which we observe some evidence. Our discovery implies that Pr2Ir2O7 is a parent state that can be manipulated to produce other strongly correlated topological phases, such as topological Mott insulator, Weyl semimetal, and quantum spin and anomalous Hall states.
The origin of superconductivity in the iron pnictides has been attributed to antiferromagnetic spin ordering that occurs in close combination with a structural transition, but there are also proposals that link superconductivity to orbital ordering. We used bulk-sensitive laser angle-resolved photoemission spectroscopy on BaFe(2)(As(0.65)P(0.35))(2) and Ba(0.6)K(0.4)Fe(2)As(2) to elucidate the role of orbital degrees of freedom on the electron-pairing mechanism. In strong contrast to previous studies, an orbital-independent superconducting gap magnitude was found for the hole Fermi surfaces. Our result is not expected from the superconductivity associated with spin fluctuations and nesting, but it could be better explained invoking magnetism-induced interorbital pairing, orbital fluctuations, or a combination of orbital and spin fluctuations. Regardless of the interpretation, our results impose severe constraints on theories of iron pnictides.
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