Liquid crystals (LCs) are soft but smart materials that can adjust its chemical or physical properties in response to various external stimuli. Using these materials to construct soft actuators and robots, referred as LC actuators and robots, is expected to replace current machinery part, obtaining lighter and smaller equipment with adjustable and complex functions. Especially, combining these LC actuator and robots with existing virtual reality and augmented reality technologies will produce a new world of mixed reality (MR) with the visual, auditory, and somatosensory interaction. In this review, the recent work on responsive LC actuators and robots is introduced, emphasizing on their potentials in haptic use. By discussing their programmable control via suitable stimuli, the LC actuators and robots are summarized for mechanical outputs, environmental mimic, and fine‐tuning of surface texture and roughness. It is anticipated that the continuous development on LC actuators and robots will accelerate the MR technology toward practical application.

Photoresponsive materials offer local, temporal, and remote control over their chemical or physical properties under external stimuli, giving new tools for interfacial regulation. Among all, photodeformable azobenzene-containing liquid crystal polymers (azo-LCPs) have received increasing attention because they can be processed into various micro/nanostructures and have the potential to reversibly tune the interfacial properties through chemical and/or morphological variation by light, providing effective dynamic interface regulation. In this feature article, we highlight the milestones in the dynamic regulation of different interfacial properties through micro/nanostructures made of photodeformable azobenzene-containing liquid crystal polymers (azo-LCPs). We describe the preparation of different azo-LCP micro/nanostructures from the aspects of materials and processing techniques and reveal the importance of mesogen orientation toward dynamic interfacial regulation. By introducing our recently developed linear azo-LCP (azo-LLCP) with good mechanical and photoresponsive performances, we discuss the challenge and opportunity with respect to the dynamic light regulation of two- and three-dimensional (2D/3D) micro/nanostructures to tune their related interfacial properties. We have also given our expectation toward exploring photodeformable micro/nanostructures for advanced applications such as in microfluidics, biosensors, and nanotherapeutics.

365 nm UV light at desired position for 300 s. The recovery of POTSMP from TS2 to PS was under the irradiation of 150 mW cm −2 , 365 nm UV light. The sample after each shape recovery could be irradiated by 80 mW cm −2 , 530 nm visible light for 3 min to recover POTSMP from cis-form to trans-form.

N-GQDs are synthesized using a simple and fast one-step protocol and applied for preparing quick-dry fluorescent ink for both writing and printing.