Quadrant analysis has been widely used to investigate the turbulent characteristics in the atmospheric boundary layer (ABL). Although quadrant analysis can identify turbulent structures that contribute significantly to turbulent fluxes, the approach to the hyperbolic hole and its parameter, referred to as hole size, remains uncertain and varies among different studies. This study discusses an improved quadrant analysis with an objective definition of the hole size for the isolation of large coherent structures from small-scale background fluctuations. Eddy covariance data collected 50 m above the grass canopy were used to analyze and evaluate the proposed method. This improved quadrant analysis ensures that the detected large coherent eddies play a dominant role in transporting fluxes, occupying 10% of the total time, with mean flux contributions ranging from 62% to 95% for momentum and 35–104% for scalars. The separated background small-scale eddies are isotropically characterized by a comparable time duration and flux contributions in each quadrant. It is observed that under an unstable atmosphere, large-scale ejections are more active than sweeps, while under stable conditions, they are equally important. Furthermore, mechanical-driven transport under near-neutral conditions only enhances ejection and sweep motions of momentum. In contrast, the buoyancy-driven scenarios under unstable conditions enhance the large-scale activities of sensible heat alone.