A highly stretchable, low-cost strain sensor was successfully prepared using an extremely cost-effective ionic liquid of ethylene glycol/sodium chloride. The hysteresis performance of the ionic-liquid-based sensor was able to be improved by introducing a wavy-shaped fluidic channel diminishing the hysteresis by the viscoelastic relaxation of elastomers. From the simulations on visco-hyperelastic behavior of the elastomeric channel, we demonstrated that the wavy structure can offer lower energy dissipation compared to a flat structure under a given deformation. The resistance response of the ionic-liquid-based wavy (ILBW) sensor was fairly deterministic with no hysteresis, and it was well-matched to the theoretically estimated curves. The ILBW sensors exhibited a low degree of hysteresis (0.15% at 250%), low overshoot (1.7% at 150% strain), and outstanding durability (3000 cycles at 300% strain). The ILBW sensor has excellent potential for use in precise and quantitative strain detections in various areas, such as human motion monitoring, healthcare, virtual reality, and smart clothes.
Flexible
and wearable pressure sensors have attracted a tremendous
amount of attention due to their wider applications in human interfaces
and healthcare monitoring. However, achieving accurate pressure detection
and stability against external stimuli (in particular, bending deformation)
over a wide range of pressures from tactile to body weight levels
is a great challenge. Here, we introduce an ultrawide-range, bending-insensitive,
and flexible pressure sensor based on a carbon nanotube (CNT) network-coated
thin porous elastomer sponge for use in human interface devices. The
integration of the CNT networks into three-dimensional microporous
elastomers provides high deformability and a large change in contact
between the conductive CNT networks due to the presence of micropores,
thereby improving the sensitivity compared with that obtained using
CNT-embedded solid elastomers. As electrical pathways are continuously
generated up to high compressive strain (∼80%), the pressure
sensor shows an ultrawide pressure sensing range (10 Pa to 1.2 MPa)
while maintaining favorable sensitivity (0.01–0.02 kPa–1) and linearity (R
2 ∼
0.98). Also, the pressure sensor exhibits excellent electromechanical
stability and insensitivity to bending-induced deformations. Finally,
we demonstrate that the pressure sensor can be applied in a flexible
piano pad as an entertainment human interface device and a flexible
foot insole as a wearable healthcare and gait monitoring device.
Bioresorbable electronic stimulators are of rapidly growing interest as unusual therapeutic platforms, i.e., bioelectronic medicines, for treating disease states, accelerating wound healing processes and eliminating infections. Here, we present advanced materials that support operation in these systems over clinically relevant timeframes, ultimately bioresorbing harmlessly to benign products without residues, to eliminate the need for surgical extraction. Our findings overcome key challenges of bioresorbable electronic devices by realizing lifetimes that match clinical needs. The devices exploit a bioresorbable dynamic covalent polymer that facilitates tight bonding to itself and other surfaces, as a soft, elastic substrate and encapsulation coating for wireless electronic components. We describe the underlying features and chemical design considerations for this polymer, and the biocompatibility of its constituent materials. In devices with optimized, wireless designs, these polymers enable stable, long-lived operation as distal stimulators in a rat model of peripheral nerve injuries, thereby demonstrating the potential of programmable long-term electrical stimulation for maintaining muscle receptivity and enhancing functional recovery.
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