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Let Ln6,4 denote a molecular graph of linear [n] phenylene with n hexagons and n squares, and let the Möbius phenylene chain H0emMn6,4 be the graph obtained from the Ln6,4 by identifying the opposite lateral edges in reversed way. Utilizing the decomposition theorem of the normalized Laplacian characteristic polynomial, we study the normalized Laplacian spectrum of H0emMn6,4, which consists of the eigenvalues of two symmetric matrices ℒ R and ℒ Q of order 3n. By investigating the relationship between the roots and coefficients of the characteristic polynomials of the two matrices above, we obtain an explicit closed‐form formula of the multiplicative degree‐Kirchhoff index as well as the number of spanning trees of H0emMn6,4. Furthermore, we determine the limited value for the quotient of the multiplicative degree‐Kirchhoff index and the Gutman index of H0emMn6,4.

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