The spatiotemporal and especially the vertical distributions of dust aerosols play crucial roles in the climatic effect of dust aerosol. In the present study, the spatial-temporal distribution of dust aerosols over East Asia was investigated using Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) retrievals (01/2007-12/2011) from the perspective of the frequency of dust occurrence (FDO), dust top layer height (TH) and profile of aerosol subtypes. The results showed that a typical dust belt was generated from the dust source regions (the Taklimakan and Gobi Deserts), in the latitude range of 25 • N~45 • N and reaching eastern China, Japan and Korea and, eventually, the Pacific Ocean. High dust frequencies were found over the dust source regions, with a seasonal sequence from high to low as follows: spring, summer, autumn and winter. Vertically, FDOs peaked at about 2 km over the dust source regions. In contrast, FDOs decreased with altitude over the downwind regions. On the dust belt from dust source regions to downwind regions, the dust top height (TH) was getting higher and higher. The dust TH varied in the range of 1.9-3.1 km above surface elevation (a.s.e.), with high values over the dust source regions and low values in the downwind areas, and a seasonally descending sequence of summer, spring, autumn and winter in accord with the seasonal variation of the boundary layer height. The annual AOD (Aerosol Optical Depth) was generally characterized by two high and two low AOD centers over East Asia. The percent contribution of the Dust Aerosol Optical Depth to the total AOD showed a seasonal variation from high to low as follows: spring, winter, autumn and summer. The vertical profile of the extinction coefficient revealed the predominance of pure dust particles in the dust source regions and a mixture of dust particles and pollutants in the downwind regions. The dust extinction coefficients over the Taklimakan Desert had a seasonal pattern from high to low as follows: spring, winter, summer and autumn. The results of the present study offered an understanding of the horizontal and vertical structures of dust aerosols over East Asia and can be used to evaluate the performance aerosol transport models.
Freezing rain has been normally considered to be composed of supercooled raindrops when the 2 m air temperature (hereafter Tas ${T}_{as}$) is below freezing. However, according to a statistical survey of freezing rain observations in China from 2000 to 2019, we find that there were 656 events that occurred at Tas ${T}_{as}$ greater than 0°C (hereafter warm freezing rain and denoted by WFR), which account for 7% of the total freezing rain observations. Additionally, nearly 3% (266 observations) of freezing rain events occurred when the near‐surface wet‐bulb temperature was greater than 0°C. The modeling and sensitivity experiments on the nonequilibrium raindrop temperature (hereafter Tr ${T}_{r}$) show that the temperature difference between raindrops and the atmosphere is the main cause of WFR. The magnitudes of the normalΔTar ${\Delta}{T}_{ar}$ (difference between raindrop temperature Tr ${T}_{r}$ and air temperature Ta ${T}_{a}$) and normalΔTwr ${\Delta}{T}_{wr}$ (difference between Tr ${T}_{r}$ and wet‐bulb temperature Tw ${T}_{w}$) are determined by the raindrop diameter D, temperature lapse rate Г, and relative humidity RH. Increases of D and Г, and a decrease of RH enhance normalΔTar ${\Delta}{T}_{ar}$ and normalΔTwr ${\Delta}{T}_{wr}$ and thus the occurrence of WFR. Further simulations of 4 idealized and 370 real sounding profiles reveal that either the Ta ${T}_{a}$ or the Tw ${T}_{w}$ cannot properly distinguish the WFR events. When considering the temperature difference between raindrops and the atmosphere, the WFR can form by the “melting of solid hydrometeors” or “supercooled warm rain process.” This study can also deepen our understanding of the conditions of WFR and freezing rain formation at different altitudes.
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