Wearable and stretchable sensors are important components to strictly monitor the behavior and health of humans and attract extensive attention. However, traditional sensors are designed with pure horseshoes or chiral metamaterials, which restrict the biological tissue engineer applications due to their narrow regulation ranges of the elastic modulus and the poorly adjustable Poisson’s ratio. Inspired by the biological spiral microstructure, a dual-phase metamaterial (chiral-horseshoes) is designed and fabricated in this work, which possesses wide and programmable mechanical properties by tailoring the geometrical parameters. Experimental, numerical, and theoretical studies are conducted, which reveal that the designed microstructures can reproduce mechanical properties of most natural animals such as frogs, snakes, and rabbits skin. Furthermore, a flexible strain sensor with the gauge factor reaching 2 under 35% strain is fabricated, which indicates that the dual-phase metamaterials have a stable monitoring ability and can be potentially applied in the electronic skin. Finally, the flexible strain sensor is attached on the human skin, and it can successfully monitor the physiological behavior signals under various actions. In addition, the dual-phase metamaterial could combine with artificial intelligence algorithms to fabricate a flexible stretchable display. The dual-phase metamaterial with negative Poisson’s ratio could decrease the lateral shrinkage and image distortion during the stretching process. This study offers a strategy for designing the flexible strain sensors with programmable, tunable mechanical properties, and the fabricated soft and high-precision wearable strain sensor can accurately monitor the skin signals under different human motions and potentially be applied for flexible display.

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